定量平面激光诱导荧光技术

Zhen Yang, Xin Yu, Jiangbo Peng, Jianlong Zhang
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引用次数: 2

摘要

平面激光诱导荧光(PLIF)是一种高灵敏度、高时空分辨的激光诊断技术。它广泛应用于燃烧和流场的诊断,以获得火焰中有效成分和感兴趣分子的热力学信息。目前,PLIF技术正朝着高速和定量化两个方向发展。鉴于PLIF技术具有其他激光诊断所不具备的高时空分辨率特点,本章将重点介绍激光诱导荧光的基本原理以及定量PLIF技术的研究现状。此外,分析了基于激光诱导荧光技术的各种火焰组分浓度定量技术的优缺点。最后介绍了利用平面激光诱导荧光定量燃烧中物质浓度的最新研究进展。为了验证修正后的测量方程的有效性,分别测量了q1(8)线(0,0)波段和(1,0)波段对OH自由基的有效峰吸收截面。实验结果表明,(0,0)波段q1(8)线OH有效峰吸收截面比(1,0)波段高约5.5倍,而LIFBASE模拟给出的理论计算值约为6倍。实验结果与仿真结果吻合较好。综述了目前火焰中物种浓度测量的PLIF定量技术的不足。介绍了利用PLIF定量测定燃烧过程中物质浓度的最新研究成果。详细介绍了一种不受碰撞淬火效应影响的非校准定量PLIF技术——双向PLIF。由于发现现有的Versluis等人提供的有效峰吸收截面测量方程不适用于弱吸收的情况,实验用方程研究了甲烷/空气部分预混火焰中OH浓度随当量比变化的二维空间分布。在0.7 -等比值下的实验结果与数值模拟结果的比较表明,双向测得的OH浓度分布与由
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Quantitative Planar Laser-Induced Fluorescence Technology
Planar laser-induced fluorescence (PLIF) is a highly sensitive and space-time-resolved laser diagnostic technique. It is widely used in the diagnosis of combustion and flow fields to obtain the thermodynamic information of active components and interested molecules in flames. Nowadays, the PLIF technology is developing in two directions: high speed and quantification. In view of the high spatial and temporal resolution characteristics of PLIF technology that other laser diagnostics do not possess, this chapter will focus on the basic principle of laser-induced fluorescence and the current research status of quantitative PLIF technology. In addition, the advantages and disadvantages of various quantitative technologies of component concentration in flames based on laser-induced fluorescence technology are analyzed. At last, the latest works on the quantification of species concentration using planar laser-induced fluorescence in combustion are introduced. confirm the validity of the modified measurement equation, the effective peak absorption cross section of the band (0,0) and band (1,0) within the Q 1 (8) line for the OH radical is measured, respectively. The experimental results show that the OH effective peak absorption cross section of the Q 1 (8) line for band (0,0) turns out to be about 5.5 times higher than that of band (1,0), while the theoretical calculation given by the LIFBASE simulation is about 6 times. The experimental result has been proven to be in good agreement with the simulation results. and disadvantages of current quantitative PLIF technologies for species concentration measurements in flames are reviewed. the latest works on the quantification of species concentration using PLIF in combustion are introduced. a non-calibration quantitative PLIF technology, named bidirectional PLIF, which is independent of collisional quenching effect, has been introduced in detail. As the current measurement equation of effective peak absorption cross section provided by Versluis et al. is found to be not applicable to the case of weak absorption, experimental equation the two-dimensional spatial distributions of OH concentration its variations with the equivalence ratios investigated in the methane/air partially premixed flame. comparison between the experimental OH concentrations and the numerical simulation results under the equivalence ratios of 0.7 – indicates the OH concentration profiles measured by bidirectional in good agreement with the predictive values performed by
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