基于设计薄膜的完美光吸收及其在结构着色、气体传感和光热转换中的应用(会议报告)

Mohamed El Kabbash, T. Letsou, M. Hinczewski, G. Strangi, Chunlei Guo
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引用次数: 0

摘要

完美光吸收(PLA)在纳米光子学中有着广泛的应用,从基于太阳热的应用到辐射冷却。然而,大多数提出的平台都需要高度光刻,这使得它们的实际意义不大。另一方面,基于成熟的技术,薄膜光吸收剂无需光刻,可以廉价地大面积沉积。然而,薄膜光吸收剂被认为有很大的局限性,无法与超材料相比进行定制。在这里,我们展示了如何使用薄膜在波长范围、带宽、光学损耗的空间分布、方向性和虹彩方面设计PLA。我们还表明,当金属具有低反射率和高折射率的氧化物时,通过简单加热金属薄膜可以产生无虹彩的PLA。从理论上和实验上论证了薄膜光吸收体中的广义布鲁斯特角效应。此外,我们使用三种不同的PLA策略演示了氢传感,显示了创纪录的灵敏度和优异值。此外,我们展示了各种策略来创造超纯的结构颜色。最后,我们展示了新型薄膜PLA设计的不同太阳能热应用。
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Designer thin-film based perfect light absorption and its applications in structural coloring, gas sensing, and solar-thermal conversion (Conference Presentation)
Perfect light absorption (PLA) in nanophotonics has a wide range of applications from solar-thermal based applications to radiative cooling. However, most of the proposed platforms require intense lithography which makes them of minor practical relevance. On the other hand, thin-film light absorbers are lithographically free and can be deposited cheaply on large area based on matured technologies. However, thin-film light absorbers were thought to have major limitation and cannot be tailored compared to metamaterials. Here, we show how to design PLA using thin-films in terms of wavelength range, bandwidth, spatial profile of optical losses, directionality and iridescence. We also show that iridescent free, PLA can occur by simply heating metallic thin-films when the metal is of low reflectance and its oxide is of high refractive index. We theoretically and experimentally demonstrate Generalized Brewster angle effect in thin film light absorbers. In addition, we demonstrate hydrogen sensing using three different PLA strategies showing record sensitivity and figure of merit. Furthermore, we show various strategies to create ultra-pure structural colors. Finally, we demonstrate different solar-thermal applications for novel thin-film PLA designs.
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