{"title":"利用飞秒激光脉冲研究暴露于α后CR-39聚合物的非线性光学性质","authors":"mona ali, M. F. Eissa, Tarek Hassan","doi":"10.1364/josab.501523","DOIUrl":null,"url":null,"abstract":"The effect of alpha particle radiation on nonlinear optical properties of poly(allyl diglycol carbonate) (CR-39) polymer has been investigated using the Z-scan technique. CR-39 polymers were exposed to alpha particles at different doses: 23.7 and 47.5 Gy. Alpha particles cause significant optical and chemical changes in the polymer CR-39. Data from UV-visible spectrometers revealed that when alpha particle doses increased, the absorption edge of polymer redshifted and the energy band gap decreased. Fourier transform infrared absorption spectra of alpha irradiation samples show a change in intensity and bond breakage in the chemical groups constituting the CR-39 polymer compared to the pristine one. With 100 fs laser pulses and 80 MHz repetition rate, the nonlinear absorption coefficient and nonlinear refractive index are measured for a pristine and irradiated polymer with different alpha doses at different excitation wavelengths and laser peak power. The samples displayed a negative nonlinear refractive index and reverse saturable absorption behavior with three photons absorption. The results reveal that the nonlinear optical properties of CR-39 were enhanced by alpha particle radiation.","PeriodicalId":17280,"journal":{"name":"Journal of The Optical Society of America B-optical Physics","volume":null,"pages":null},"PeriodicalIF":1.8000,"publicationDate":"2023-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Using Femtosecond Laser Pulses to Explore the Nonlinear Optical Properties of a CR-39 Polymer after being Exposed to Alpha\",\"authors\":\"mona ali, M. F. Eissa, Tarek Hassan\",\"doi\":\"10.1364/josab.501523\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The effect of alpha particle radiation on nonlinear optical properties of poly(allyl diglycol carbonate) (CR-39) polymer has been investigated using the Z-scan technique. CR-39 polymers were exposed to alpha particles at different doses: 23.7 and 47.5 Gy. Alpha particles cause significant optical and chemical changes in the polymer CR-39. Data from UV-visible spectrometers revealed that when alpha particle doses increased, the absorption edge of polymer redshifted and the energy band gap decreased. Fourier transform infrared absorption spectra of alpha irradiation samples show a change in intensity and bond breakage in the chemical groups constituting the CR-39 polymer compared to the pristine one. With 100 fs laser pulses and 80 MHz repetition rate, the nonlinear absorption coefficient and nonlinear refractive index are measured for a pristine and irradiated polymer with different alpha doses at different excitation wavelengths and laser peak power. The samples displayed a negative nonlinear refractive index and reverse saturable absorption behavior with three photons absorption. The results reveal that the nonlinear optical properties of CR-39 were enhanced by alpha particle radiation.\",\"PeriodicalId\":17280,\"journal\":{\"name\":\"Journal of The Optical Society of America B-optical Physics\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2023-10-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of The Optical Society of America B-optical Physics\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1364/josab.501523\",\"RegionNum\":4,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of The Optical Society of America B-optical Physics","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1364/josab.501523","RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"OPTICS","Score":null,"Total":0}
Using Femtosecond Laser Pulses to Explore the Nonlinear Optical Properties of a CR-39 Polymer after being Exposed to Alpha
The effect of alpha particle radiation on nonlinear optical properties of poly(allyl diglycol carbonate) (CR-39) polymer has been investigated using the Z-scan technique. CR-39 polymers were exposed to alpha particles at different doses: 23.7 and 47.5 Gy. Alpha particles cause significant optical and chemical changes in the polymer CR-39. Data from UV-visible spectrometers revealed that when alpha particle doses increased, the absorption edge of polymer redshifted and the energy band gap decreased. Fourier transform infrared absorption spectra of alpha irradiation samples show a change in intensity and bond breakage in the chemical groups constituting the CR-39 polymer compared to the pristine one. With 100 fs laser pulses and 80 MHz repetition rate, the nonlinear absorption coefficient and nonlinear refractive index are measured for a pristine and irradiated polymer with different alpha doses at different excitation wavelengths and laser peak power. The samples displayed a negative nonlinear refractive index and reverse saturable absorption behavior with three photons absorption. The results reveal that the nonlinear optical properties of CR-39 were enhanced by alpha particle radiation.
期刊介绍:
The Journal of the Optical Society of America B (JOSA B) is a general optics research journal that complements JOSA A. It emphasizes scientific research on the fundamentals of the interaction of light with matter such as quantum optics, nonlinear optics, and laser physics. Topics include:
Advanced Instrumentation and Measurements
Fiber Optics and Fiber Lasers
Lasers and Other Light Sources from THz to XUV
Light-Induced Phenomena
Nonlinear and High Field Optics
Optical Materials
Optics Modes and Structured Light
Optomechanics
Metamaterials
Nanomaterials
Photonics and Semiconductor Optics
Physical Optics
Plasmonics
Quantum Optics and Entanglement
Quantum Key Distribution
Spectroscopy and Atomic or Molecular Optics
Superresolution and Advanced Imaging
Surface Optics
Ultrafast Optical Phenomena
Wave Guiding and Optical Confinement
JOSA B considers original research articles, feature issue contributions, invited reviews and tutorials, and comments on published articles.