二维摩尔超晶格中的非线性霍尔效应

None Zefei Wu, None Meizhen Huang, None Ning Wang
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Experimentally, when a longitudinal ac electric field is applied, a transvers Hall voltage will be generated, with its amplitude proportional to the square of the driving current. Such nonlinear Hall signal contains two components: one is an ac transverse voltage that oscillates at a frequency that twice of the driving current, and the other is a DC signal converted from the injected current. Although the history of the nonlinear Hall effect is only a few years, its broad application prospects in the fields of wireless communication, energy harvesting, and infrared detectors have been widely recognized. The main reason is that the frequency doubling and rectification of electrical signals via the nonlinear Hall effect are achieved by the inherent quantum properties of the material - the Berry curvature dipole moment, and therefore do not have the thermal voltage thresholds and/or the transition time characteristic of semiconductor junctions/diodes. Unfortunately, the existence of the Berry curvature dipole moment has more stringent requirements on the lattice symmetry of the system in addition to the space inversion breaking, and the available materials are very limited. This greatly reduces the chance to optimize the signal of the nonlinear Hall effect and limits the application and development of the nonlinear Hall effect. The rapid development of van der Waals stacking technology in recent years provides a new way to design, tailor and control the symmetry of lattice, and prepare artificial moiré crystals with certain physical properties. Recently, both theoretical and experimental studies on graphene superlattices and transition metal chalcogenide superlattices have shown that artificial moiré superlattice materials can have larger Berry curvature dipole moments than natural non-moiré crystals, which has obvious advantages in generating and manipulating the nonlinear Hall effect. On the other hand, abundant strong correlation effects have been observed in two dimensional superlattices. The study of the nonlinear Hall effect in two-dimensional moiré superlattices can not only give people a new understanding of the momentum space distribution of Berry curvatures, contributing to the realization of more stable topological transport, correlation insulating state and superfluidity state, but also expand the functional space of moiré superlattice materials which are promising for the design of new electronic and optoelectronic devices. This review paper firstly introduces the birth and development of the nonlinear Hall effect and discusses the two mechanism of the nonlinear Hall effects: Berry curvature dipole moment and disorder. 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引用次数: 0

摘要

霍尔效应是指在垂直于施加电流的方向上产生电压。霍尔效应家族自1879年被发现以来,已成为一个庞大的群体,对其深入研究是凝聚态物理领域的一个重要课题。新发现的非线性霍尔效应是霍尔效应的新成员。与以往的大多数霍尔效应不同,非线性霍尔效应不需要打破系统的时间反转对称性,但需要空间反转不对称性。自2015年以来,非线性霍尔效应被预测并证实存在于几种能带Berry曲率分布不均匀的材料中。实验表明,当施加纵向交流电场时,将产生横向霍尔电压,其幅值与驱动电流的平方成正比。这种非线性霍尔信号包含两个分量:一个是以驱动电流两倍的频率振荡的交流横向电压,另一个是由注入电流转换而成的直流信号。虽然非线性霍尔效应的研究历史只有短短几年,但其在无线通信、能量采集、红外探测器等领域的广阔应用前景已得到广泛认可。主要原因是,通过非线性霍尔效应实现的电信号的倍频和整流是由材料固有的量子特性-贝里曲率偶极矩实现的,因此不具有半导体结/二极管的热电压阈值和/或过渡时间特性。遗憾的是,Berry曲率偶极矩的存在除了空间反转破缺外,对系统的晶格对称性有更严格的要求,而且可用的材料非常有限。这大大减少了非线性霍尔效应信号优化的机会,限制了非线性霍尔效应的应用和发展。近年来范德华叠加技术的迅速发展为设计、裁剪和控制晶格的对称性,制备具有一定物理性质的人工莫尔瓦晶体提供了新的途径。近年来,对石墨烯超晶格和过渡金属硫系化合物超晶格的理论和实验研究表明,人工莫尔晶格材料比天然非莫尔晶格具有更大的Berry曲率偶极矩,在产生和操纵非线性霍尔效应方面具有明显的优势。另一方面,在二维超晶格中观察到大量的强相关效应。二维moir超晶格中非线性霍尔效应的研究,不仅使人们对Berry曲率的动量空间分布有了新的认识,有助于实现更稳定的拓扑输运、相关绝缘态和超流体态,而且拓展了moir超晶格材料的功能空间,为新型电子和光电子器件的设计提供了前景。本文首先介绍了非线性霍尔效应的产生和发展,讨论了非线性霍尔效应的两种机制:贝里曲率偶极矩和无序。随后,本文总结了二维莫尔维尔超晶格实现非线性霍尔效应所必需的一些性质:可观的贝里曲率、对称性破缺、强相关效应和可调谐的能带结构。其次,综述了石墨烯和过渡金属硫族化物超晶格中非线性霍尔效应的理论和实验进展。最后,展望了基于摩尔超晶格材料的非线性霍尔效应的未来研究方向和潜在应用。
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The nonlinear Hall effect in two dimensional moiré superlattices
The Hall effect refers to the generation of a voltage in a direction perpendicular to the applied current. Since its discovery in 1879, the Hall effect family has become a huge group, and its in-depth study is an important topic in the field of condensed matter physics. The newly discovered nonlinear Hall effect is a new member of the Hall effects. Unlike most of the previous Hall effects, the nonlinear Hall effect does not need to break the time-reversal symmetry of the system but requires the spatial inversion asymmetry. Since 2015, the nonlinear Hall effect has been predicted and confirmed to exist in several kinds of materials with nonuniform distribution of Berry curvature of the energy bands. Experimentally, when a longitudinal ac electric field is applied, a transvers Hall voltage will be generated, with its amplitude proportional to the square of the driving current. Such nonlinear Hall signal contains two components: one is an ac transverse voltage that oscillates at a frequency that twice of the driving current, and the other is a DC signal converted from the injected current. Although the history of the nonlinear Hall effect is only a few years, its broad application prospects in the fields of wireless communication, energy harvesting, and infrared detectors have been widely recognized. The main reason is that the frequency doubling and rectification of electrical signals via the nonlinear Hall effect are achieved by the inherent quantum properties of the material - the Berry curvature dipole moment, and therefore do not have the thermal voltage thresholds and/or the transition time characteristic of semiconductor junctions/diodes. Unfortunately, the existence of the Berry curvature dipole moment has more stringent requirements on the lattice symmetry of the system in addition to the space inversion breaking, and the available materials are very limited. This greatly reduces the chance to optimize the signal of the nonlinear Hall effect and limits the application and development of the nonlinear Hall effect. The rapid development of van der Waals stacking technology in recent years provides a new way to design, tailor and control the symmetry of lattice, and prepare artificial moiré crystals with certain physical properties. Recently, both theoretical and experimental studies on graphene superlattices and transition metal chalcogenide superlattices have shown that artificial moiré superlattice materials can have larger Berry curvature dipole moments than natural non-moiré crystals, which has obvious advantages in generating and manipulating the nonlinear Hall effect. On the other hand, abundant strong correlation effects have been observed in two dimensional superlattices. The study of the nonlinear Hall effect in two-dimensional moiré superlattices can not only give people a new understanding of the momentum space distribution of Berry curvatures, contributing to the realization of more stable topological transport, correlation insulating state and superfluidity state, but also expand the functional space of moiré superlattice materials which are promising for the design of new electronic and optoelectronic devices. This review paper firstly introduces the birth and development of the nonlinear Hall effect and discusses the two mechanism of the nonlinear Hall effects: Berry curvature dipole moment and disorder. Subsequently, this paper summaries some properties of two-dimensional moiré superlattices which are essential in realizing the nonlinear Hall effect: considerable Berry curvature, symmetry breaking, strong correlation effect and tunable band structure. Next, this paper reviews the theoretical and experimental progress of the nonlinear Hall effects in graphene and transition metal chalcogenide superlattices. Finally, the future research directions and potential applications of the nonlinear Hall effect based on moiré superlattice materials are prospected.
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