平面预混火焰与剪切流对齐的扩散热不稳定性

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2023-09-20 DOI:10.1080/13647830.2023.2254734
Joel Daou, Prabakaran Rajamanickam
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引用次数: 1

摘要

研究了厚平面预混火焰沿单向剪切流横向稳定传播的稳定性。在无限大活化能的渐近极限下进行了线性稳定性分析,得到了色散关系。该关系通过两个主要参数,即反应物路易斯数Le和流动佩莱特数Pe,表征了泰勒弥散(或剪切增强扩散)与火焰热扩散不稳定性之间的耦合。讨论了色散关系的含义,并在Le-Pe平面上对各种火焰不稳定性进行了识别和分类。一个重要的原始发现是证明,对于超过临界值的佩莱特数值,经典的细胞不稳定性,通常在Le1中发现,但当Le1显示通过有限波长平稳分岔(也称为i型)或通过长波平稳分岔(也称为ii型)发生时不存在。后一类分岔导致弱非线性区域的Kuramoto-Sivashinsky方程,该方程是确定的。对于振荡不稳定性,通常在Le>1混合物中没有Taylor色散时遇到,如果Peclet数足够大,则发现不存在振荡不稳定性。稳定性的发现,从色散关系推导出的解析,补充和数值检验了有限值的Zeldovich数。数值研究包括线性稳定性边值问题的特征值计算和时变控制偏微分方程的数值模拟。计算结果与分析预测结果在定性上是一致的。
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Diffusive-thermal instabilities of a planar premixed flame aligned with a shear flow
The stability of a thick planar premixed flame, propagating steadily in a direction transverse to that of unidirectional shear flow, is studied. A linear stability analysis is carried out in the asymptotic limit of infinitely large activation energy, yielding a dispersion relation. The relation characterises the coupling between Taylor dispersion (or shear-enhanced diffusion) and the flame thermo-diffusive instabilities, in terms of two main parameters, namely, the reactant Lewis number Le and the flow Peclet number Pe. The implications of the dispersion relation are discussed and various flame instabilities are identified and classified in the Le-Pe plane. An important original finding is the demonstration that for values of the Peclet number exceeding a critical value, the classical cellular instability, commonly found for Le<1, exists now for Le>1 but is absent when Le<1. In fact, the cellular instability identified for Le>1 is shown to occur either through a finite-wavelength stationary bifurcation (also known as type-Is) or through a longwave stationary bifurcation (also known as type-IIs). The latter type-IIs bifurcation leads in the weakly nonlinear regime to a Kuramoto-Sivashinsky equation, which is determined. As for the oscillatory instability, usually encountered in the absence of Taylor dispersion in Le>1 mixtures, it is found to be absent if the Peclet number is large enough. The stability findings, which follow from the dispersion relation derived analytically, are complemented and examined numerically for a finite value of the Zeldovich number. The numerical study involves both computations of the eigenvalues of a linear stability boundary-value problem and numerical simulations of the time-dependent governing partial differential equations. The computations are found to be in good qualitative agreement with the analytical predictions.
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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