不对称双分裂环谐振器元表面中的窄线宽圆二色性

Liangkun Dai, Chengchen Bi, Lu Chen, Zhaomin Rong, Wu Fei, Xiangyun Jiang, Chan Huang, Jigang Hu
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摘要

强窄线宽圆二色性(CD)光谱有望应用于生物化学传感和天然分子中弱手性的检测。在此,我们提出了一种由不对称金属双分裂环谐振器(DSRR)阵列形成的手性元表面,并对其圆二色性(CD)进行了研究。该元表面吸收响应的最大 CD 值可达 0.61,在中红外(MIR)波段的超窄光谱线宽为 9.6 nm。计算结果表明,手性元表面可支持左圆极化(LCP)和右圆极化(RCP)光的两种表面晶格共振模式。自旋选择性高 Q 值共振模式对左旋偏振光和右旋偏振光具有不同的吸收率,从而实现了 CD 的窄线宽。我们的发现揭示了自旋选择性完美光吸收、高灵敏度偏振检测和手性传感的潜在应用。
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Narrow-linewidth circular dichroism in asymmetric double split ring resonator metasurface
Strong and narrow-linewidth circular dichroism (CD) spectroscopy promises potential applications in bio-chemical sensing and detection of the weak chirality in natural molecules. Here we proposed a chiral metasurface formed by the asymmetric metal double split ring resonator (DSRR) arrays, the circular dichroism (CD) of which has been investigated. The maximum CD for absorption response of the metasurface can reach 0.61 with an ultra-narrow spectral linewidth of 9.6 nm in the mid-infrared (MIR) band. Our calculation results show that the chiral metasurface can support two surface lattice resonance modes for the left circularly polarized (LCP) and right circularly polarized (RCP) light. The narrow linewidth of CD is enabled by the spin-selective high-Q resonance modes with a differential absorptivity for LCP and RCP light. Our findings shed light on the potential applications in spin-selective perfect optical absorption, high-sensitive polarization detection, and chirality sensing.
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