超声波增强过硫酸盐氧化系统对新出现污染物的净化作用

IF 10.7 1区 工程技术 Q1 CHEMISTRY, PHYSICAL Green Energy & Environment Pub Date : 2024-01-14 DOI:10.1016/j.gee.2024.01.004
Yanpan Li, Yanbo Zhou, Yi Zhou
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引用次数: 0

摘要

新出现的污染物(ECs)广泛存在于水生环境中,对生态系统和人类健康构成潜在风险。超声波辅助的过硫酸盐氧化过程能够同时产生硫酸根自由基和空化效应,增强降解效果,因此在降解 ECs 方面备受关注。本文综述了超声协同类 Fenton 氧化系统降解有机污染物的原理,分为均相系统、非均相系统和单原子系统三个方面探讨了超声增强过硫酸盐技术的协同效应,并讨论了超声频率和功率、系统 pH 值、温度、初始氧化剂浓度等环境因素对系统去污性能的影响。最后,对超声波活化过硫酸盐技术的未来研究进行了总结和展望。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Ultrasonic enhancement of persulfate oxidation system governs emerging pollutants decontamination

Emerging contaminants (ECs) are widely present in aquatic environments, posing potential risks to both ecosystems and human health. The ultrasound-assisted persulfate oxidation process has attracted considerable attention in the degradation of ECs due to its ability to generate both sulfate radicals and cavitation effects, enhancing degradation effects. In this paper, the principle of ultrasonic synergistic Fenton-like oxidation system for degrading organic pollutants was reviewed, divided into homogeneous system, non-homogeneous system, and single-atom system to explore the synergistic effect of ultrasound-enhanced persulfate technology in three aspects, and the effects of environmental factors such as ultrasonic frequency and power, system pH, temperature, and initial oxidant concentration on the system's decontamination performance were discussed. Finally, future research on ultrasonically activated persulfate technology is summarized and prospected.

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来源期刊
Green Energy & Environment
Green Energy & Environment Energy-Renewable Energy, Sustainability and the Environment
CiteScore
16.80
自引率
3.80%
发文量
332
审稿时长
12 days
期刊介绍: Green Energy & Environment (GEE) is an internationally recognized journal that undergoes a rigorous peer-review process. It focuses on interdisciplinary research related to green energy and the environment, covering a wide range of topics including biofuel and bioenergy, energy storage and networks, catalysis for sustainable processes, and materials for energy and the environment. GEE has a broad scope and encourages the submission of original and innovative research in both fundamental and engineering fields. Additionally, GEE serves as a platform for discussions, summaries, reviews, and previews of the impact of green energy on the eco-environment.
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