使用 Mann-Kendall 和小波相干性方法分析撒哈拉以南高污染地区的夜间气溶胶及其与协变量的关系。

IF 2.2 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Journal of environmental quality Pub Date : 2024-01-31 DOI:10.1002/jeq2.20543
Ali Köse, Salman Tariq, Banu Numan Uyal, Muhammad Khan, Husam Rjoub, Usman Mehmood
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引用次数: 0

摘要

夜间气溶胶和痕量气体的大量排放会导致严重的空气质量、气候和健康问题,尤其是在污染严重的城市。本文试图研究撒哈拉以南城市伊洛林(尼日利亚)夜间气溶胶和痕量气体的变化情况。我们使用了气溶胶机器人网络的 500 纳米气溶胶光学深度(AOD)、安氏指数(AE)(440/870)和可降水量(WVC)数据。AE和WVC均呈逐年下降趋势,降幅分别为-0.0012%和-0.0010%。我们还分析了大气红外探测器(Atmospheric Infrared Sounder)的一氧化碳(CO)、甲烷(CH4)和臭氧(O3)夜间数据,以及云-气溶胶激光雷达和红外探路者卫星观测(CALIPSO)的气溶胶子类型数据。发现 AOD、AE 和 WVC 平均值分别为 0.64 ± 0.33、0.74 ± 0.24 和 3.40 ± 0.97。由于旱季期间东北风携带撒哈拉沙尘,二月份观测到的 AOD 值最大(1.29)。沙漠尘埃气溶胶(37.63%)是最常见的类型,其次是混合气溶胶(44.15%)。离地面 1500 米高处的风可能将撒哈拉沙尘带到了伊洛林。CALIPSO 图像显示,伊洛林的大气中含有尘埃、受污染的大陆性尘埃、清洁的海洋性尘埃以及高日空气耗氧量天的受污染尘埃。美国国家海洋和大气管理局的垂直探测剖面图显示,高 AOD 值的出现是由反转层捕获气溶胶污染造成的。测得的 CO、O3 和 CH4 夜间平均浓度分别为 127 ± 18、29.7 ± 2.1 和 1822.6 ± 12.7 ppbv。小波相干谱显示出明显的准半年度和准年度振荡,在统计学上具有显著意义。
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Analysis of nighttime aerosols and relation to covariates over a highly polluted sub-Saharan site using Mann–Kendall and wavelet coherence approach

High emissions of aerosols and trace gases during nighttime can cause serious air quality, climate, and health issues, particularly in extremely polluted cities. In this paper, an effort has been made to examine the variations in aerosols and trace gases over a sub-Saharan city of Ilorin (Nigeria) during nighttime. We have used Aerosol Robotic Network data of aerosol optical depth (AOD) at 500 nm, Angstrom exponent (AE) (440/870), and precipitable water (WVC). Both AE and WVC showed a decreasing trend of −0.0012% and −0.0010% per year, respectively. We also analyzed nighttime data of carbon monoxide (CO), methane (CH4), and ozone (O3) from Atmospheric Infrared Sounder and aerosol subtypes from CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation). AOD, AE, and WVC average values are found to be 0.64 ± 0.33, 0.74 ± 0.24, and 3.40 ± 0.97, respectively. As a result of northeasterly winds carrying Saharan dust during the dry season, the greatest value of AOD (1.29) was observed in February. Desert dust aerosols (37.63%) were the most prevalent type, followed by mixed aerosols (44.15%). Winds at a height of 1500 m above ground level were likely transporting Saharan dust to Ilorin. CALIPSO images revealed that Ilorin's atmosphere contained dust, polluted continental, clean maritime, and polluted dust on high AOD days. The National Oceanic and Atmospheric Administration's vertical sounding profiles showed that the presence of high AOD values was caused by the inversion layer trapping aerosol pollution. Average nighttime concentrations of CO, O3, and CH4 were measured to be 127 ± 18, 29.7 ± 2.1, and 1822.6 ± 12.7 ppbv, respectively. The wavelet coherence spectra exhibited significant quasi-biannual and quasi-annual oscillations at statistically significant levels.

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来源期刊
Journal of environmental quality
Journal of environmental quality 环境科学-环境科学
CiteScore
4.90
自引率
8.30%
发文量
123
审稿时长
3 months
期刊介绍: Articles in JEQ cover various aspects of anthropogenic impacts on the environment, including agricultural, terrestrial, atmospheric, and aquatic systems, with emphasis on the understanding of underlying processes. To be acceptable for consideration in JEQ, a manuscript must make a significant contribution to the advancement of knowledge or toward a better understanding of existing concepts. The study should define principles of broad applicability, be related to problems over a sizable geographic area, or be of potential interest to a representative number of scientists. Emphasis is given to the understanding of underlying processes rather than to monitoring. Contributions are accepted from all disciplines for consideration by the editorial board. Manuscripts may be volunteered, invited, or coordinated as a special section or symposium.
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