基于 UiO-66(Zr)的水净化功能材料:最新综述

Environmental Functional Materials Pub Date : 2023-08-01 Epub Date: 2024-02-11 DOI:10.1016/j.efmat.2024.02.001
Yu-Hang Li, Chong-Chen Wang, Xiao-Hong Yi, Hong-Yu Chu
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引用次数: 0

摘要

UiO-66作为一种经典的金属有机骨架(MOF),因其丰富的孔隙、超大的比表面积、优异的稳定性、奇特的性能和功能,被认为是最有前途的实用水净化MOF材料之一。近年来,为了进一步增强uio -66基材料在水环境修复中的应用,包括功能改性、缺陷工程、uio -66基复合材料和膜的构建等一系列有效策略引起了研究者的广泛关注。本文综述了废水处理中各种设计策略和相应的结构-性能关系的最新进展。不同的设计策略诱导了特定的应用,包括环境催化、吸附和荧光传感检测,并通过典型作品进行了澄清。此外,还详细介绍了其机制和相应的概念验证技术。最后,提出了UiO-66基功能材料(包括原始UiO-66及其衍生物/复合材料)在污染物去除和传感检测方面存在的挑战和未来前景。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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UiO-66(Zr)-based functional materials for water purification: An updated review
UiO-66, as a kind of classic metal-organic frameworks (MOFs), was foreseen as one of the most promising MOF materials for practical water purification, benefiting from its merits of rich pores, super-huge specific surface area, outstanding stability, intriguing properties and functions. Recently, to further enhance the applications of UiO-66-based materials in water environmental restoration, series effective strategies including functional modification, defect engineering, construction of UiO-66-based composites and membranes, had captured widespread interests by researchers. In this review, the recent advances in both various design strategies and corresponding structure-property relationships in wastewater treatment were summarized. The different design strategies induced particular applications, involving environmental catalysis, adsorption and fluorescent sensing detection, had been clarified with typical works. Moreover, the mechanisms and corresponding proof-of-concept techniques were also reviewed in detail. Finally, the existing challenges and future prospects of UiO-66 based functional materials including the pristine UiO-66 and its derivatives/composites for pollutants removal and sensing detection were proposed.
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