水热法辅助合成掺锶 SnS 纳米花催化剂,用于在自然阳光照射下光降解废水中的甲硝唑抗生素污染物。

IF 2.5 4区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL Water Science and Technology Pub Date : 2024-03-01 DOI:10.2166/wst.2024.054
Tayeb Bouarroudj, Youcef Messai, Lamine Aoudjit, Beddiaf Zaidi, Djamila Zioui, Amel Bendjama, Samiha Mezrag, Abdelmounaim Chetoui, Ilyas Belkhettab, Khaldoun Bachari
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引用次数: 0

摘要

在本研究中,我们报告了一种掺锶 SnS 纳米花的简便水热合成方法,该方法可用作降解水中抗生素分子的催化剂。利用 X 射线衍射 (XRD)、扫描电子显微镜 (SEM) 和紫外可见吸收光谱 (UV-Vis) 对制备的样品进行了表征。通过研究光催化条件下水溶液中甲硝唑的降解情况,评估了掺锶 SnS 纳米花的光催化能力。在中性 pH 条件下,降解研究的反应时间为 300 分钟,结果发现甲硝唑的降解率达到 91%,表明催化剂具有优异的光催化性能。优化了催化剂用量、甲硝唑初始浓度、初始反应 pH 值和光源性质等实验参数对甲硝唑降解时间的影响。研究还考察了掺锶 SnS 纳米花催化剂的可重复使用性,其光催化效率在使用四个周期后仍保持不变。
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Hydrothermal-assisted synthesis of Sr-doped SnS nanoflower catalysts for photodegradation of metronidazole antibiotic pollutant in wastewater promoted by natural sunlight irradiation.

In this study, we report a facile hydrothermal synthesis of strontium-doped SnS nanoflowers that were used as a catalyst for the degradation of antibiotic molecules in water. The prepared sample was characterized using X-ray diffraction (XRD), scanning electron microscopy (SEM), and ultraviolet-visible absorption spectroscopy (UV-Vis). The photocatalytic ability of the strontium-doped SnS nanoflowers was evaluated by studying the degradation of metronidazole in an aqueous solution under photocatalytic conditions. The degradation study was conducted for a reaction period of 300 min at neutral pH, and it was found that the degradation of metronidazole reached 91%, indicating the excellent photocatalytic performance of the catalyst. The influence of experimental parameters such as catalyst dosage, initial metronidazole concentration, initial reaction pH, and light source nature was optimized with respect to metronidazole degradation over time. The reusability of the strontium-doped SnS nanoflowers catalyst was investigated, and its photocatalytic efficiency remained unchanged even after four cycles of use.

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来源期刊
Water Science and Technology
Water Science and Technology 环境科学-工程:环境
CiteScore
4.90
自引率
3.70%
发文量
366
审稿时长
4.4 months
期刊介绍: Water Science and Technology publishes peer-reviewed papers on all aspects of the science and technology of water and wastewater. Papers are selected by a rigorous peer review procedure with the aim of rapid and wide dissemination of research results, development and application of new techniques, and related managerial and policy issues. Scientists, engineers, consultants, managers and policy-makers will find this journal essential as a permanent record of progress of research activities and their practical applications.
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