作为木质纤维素生物质预处理方法的新型高级氧化工艺 (AOP) 及其可持续性评估:综述

IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Current Pollution Reports Pub Date : 2024-03-14 DOI:10.1007/s40726-024-00295-w
Javad Toghiani, Sajjad Malekzadeh, Neda Jamali, Neda Afsham, Narges Fallah, Amir Mahboubi, Bahram Nasernejad, Mohammad J. Taherzadeh, Sepideh Oladzad
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引用次数: 0

摘要

综述目的木质纤维素生物质作为一种绿色可持续资源,可用于生物炼制厂生产生物基产品。木质纤维素的结构复杂且具有抗性,在生物炼制的主要过程中,微生物无法获得碳水化合物,因此必须进行预处理。本综述对不同的传统预处理方法(物理、物理化学、化学和生物方法)以及新型高级氧化工艺(AOPs)及其可持续性、环境影响、经济可行性、能源效率和商业化状态进行了研究。随着对 AOPs 运行机制和原理的研究,在 AOPs 预处理方法中,羟基自由基(-OH)的产生足以通过氧化作用分解木质纤维素结构。本文综述了近期用于木质纤维素预处理的不同 AOPs,即 Fenton 工艺、臭氧氧化、光化学、湿空气氧化、超声波和电化学。此外,表中还简要介绍了不同 AOPs 预处理研究的成果和工艺操作条件的总体趋势。此外,还讨论了木质纤维素生物质预处理可持续性评估方法,如生命周期评估(LCA)和经济价值与环境影响(EVEI)。虽然没有研究对不同 AOP 与传统方法的可持续性方面进行比较,但本综述总体上讨论了这些方面。本综述深入探讨了生物炼制的瓶颈--预处理,并全面研究了 AOPs 方法的机理、工作原理、可持续性、环境、经济、能源和商业化状况。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Novel Advanced Oxidation Processes (AOPs) as Lignocellulosic Biomass Pretreatment Approaches and Their Sustainability Assessment: A Review

Purpose of Review

Lignocellulosic biomass, as a green and sustainable resource, can be used in biorefineries to produce bio-based products. The complex and resistant structure of lignocellulose prevents microorganisms access to carbohydrates in the biorefinery’s main processes, necessitating pretreatment. Different conventional pretreatment methods (physical, physico-chemical, chemical, and biological methods) and also novel advanced oxidation processes (AOPs) and their sustainability, environmental impact, economic viability, energy efficiency and, commercialization state are investigated in this review.

Recent Findings

Due to various reviews and studies on conventional pretreatment methods, they are briefly described with proper data. As the mechanisms and principle of operation of AOPs were investigated, during the AOPs pretreatment methods, hydroxyl radicals (·OH) are generated sufficiently to decompose lignocellulosic structure through oxidation. In this paper, we review the different AOPs, i.e., Fenton process, ozonation, photochemical, wet air oxidation, ultrasound, and electrochemical, which are recently used in the pretreatment of lignocellulose. Also, the achievement of different AOPs pretreatment research studies and general trends governing the process operating conditions are presented briefly in tables. Moreover, lignocellulosic biomass pretreatment sustainability assessment approaches such as life cycle assessment (LCA) and economic value and environmental impact (EVEI) are discussed. Although no study compared the sustainability aspects of different AOPs with conventional methods, this review generally addresses them. Further, environmental, energetic, and economic aspects of AOPs methods have been compared as important criteria in selecting a pretreatment method.

Summary

This review provides a thorough insight into the biorefinery’s bottleneck, pretreatment, and comprehensively investigated mechanisms, principle of operation, sustainability, environmental, economic, energy, and commercialization state of AOPs methods.

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来源期刊
Current Pollution Reports
Current Pollution Reports Environmental Science-Water Science and Technology
CiteScore
12.10
自引率
1.40%
发文量
31
期刊介绍: Current Pollution Reports provides in-depth review articles contributed by international experts on the most significant developments in the field of environmental pollution.By presenting clear, insightful, balanced reviews that emphasize recently published papers of major importance, the journal elucidates current and emerging approaches to identification, characterization, treatment, management of pollutants and much more.
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