基于二维材料的柔性一次性气体传感器

Farah Ma'ashi, A. Aljarb, H. Al‐Jawhari
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摘要

过渡金属二卤化物(TMDCs)纳米材料,尤其是二硫化钼(MoS2),因其对气体分子的极度敏感性、超强的机械和电气性能以及大表面积,已被频繁用作柔性气体传感器的基础材料。这项工作旨在研究由二维 MoS2 制成的柔性气体传感器在暴露于百万分之一(ppm)级的二氧化氮(NO2)气体时的行为。单层 MoS2 是通过化学气相沉积(CVD)法成功合成的。拉曼光谱和光致发光(PL)证实了 MoS2 层的形成。通过将两个 MoS2 样品(从 CVD 管内的两个位置获得)转移到纸基板上,制造出了两种不同的气体传感装置。具体来说,上游样品 Sup 取自靠近 MoO3 源的区域,下游样品 Sdown 取自远离 MoO3 源的区域。这两种传感器对低至 (1.5 ppm) 浓度的二氧化氮都有很好的响应。虽然 Sdown 的响应率高达 62.8%,响应速度也很快,仅需 9 秒,但传感器的恢复时间却很慢,仅需 42 秒。另一方面,Sup 表现出良好的稳定性,其响应率为 36.8%,响应时间和恢复时间分别为 20 秒和 27 秒。这种行为可归因于两种 MoS2 样品的反应性不同。这项工作为进一步改进基于 MoS2 的柔性气体传感器的制造开辟了道路。
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Flexible and Disposable Gas Sensors Based on Two-Dimensional Materials
Transition metal dichalcogenides (TMDCs) nanomaterials, in particular Molybdenum disulfide (MoS2), have been employed frequently as a basis for flexible gas sensors due to their extreme sensitivity to gas molecules, super mechanical and electrical properties, and large surface area. This work aims to study the behavior of the flexible gas sensor made of 2D-MoS2 under exposure to nitrogen dioxide (NO2) gas at the part per million (ppm) level. The mono-layered MoS2 was successfully synthesized by Chemical Vapor Deposition (CVD). The formation of MoS2 layers was confirmed by Raman spectroscopy and Photoluminescence (PL). Two different gas-sensing devices were fabricated by transferring two MoS2 samples (obtained from two positions inside the CVD tube) onto paper substrates. Specifically, upstream sample Sup was obtained from an area near the MoO3 source, and downstream sample Sdown was obtained from an area far from the MoO3 source. Both sensors showed a good response to a concentration as low as (1.5 ppm) of NO2. Although a high response of 62.8% along with a fast response of 9 sec were recorded by Sdown, the sensor showed a slow recovery time of 42 sec. On the other hand, Sup showed good stability with an appropriate response of 36.8% along with a reasonable response time and recovery times of 20 and 27 sec, respectively. Such behavior could be accredited to the difference in the reactivity in both MoS2 samples. This work opens the way for further improvements in manufacturing MoS2-based flexible gas sensors.
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