液体表面凹陷大小对等离子体-液体阳极系统中放电特性和化学分布的影响

Yun Ling, D. Dai, Jiaxin Chang, Buang Wang
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引用次数: 0

摘要

常压等离子体与液体的相互作用存在于多种应用中,包括废水处理、伤口杀菌和消毒。在实际应用中,不可避免地会出现液体表面凹陷的现象。外加气体会造成液体表面凹陷,这无疑会影响等离子体的产生,并进一步影响应用性能。然而,液体表面变形对等离子体的影响尚不清楚。本研究建立了数值模型,以揭示液面凹陷影响等离子体放电特性的机理以及随之而来的等离子体物种分布,并进一步研究了不同氦气流速产生的不同大小的液面凹陷对等离子体的影响。结果表明,液面变形改变了初始空间电场,导致液面上的电子重新排列。沉积在液体表面的电荷进一步增加了电场的畸变程度。此外,受液面凹陷影响的电场和电子分布极大地影响了活性物种的生成和分布,从而决定了相关应用的实际效果。本研究探讨了以往相关研究中被忽视的液面凹陷现象,有助于进一步理解等离子体与液体的相互作用,为相关应用和技术提供更好的理论指导。
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Effect of liquid surface depression size on discharge characteristics and chemical distribution in the plasma-liquid anode system
Atmospheric pressure plasma-liquid interactions exist in a variety of applications, including wastewater treatment, wound sterilization, and disinfection. In practice, the phenomenon of liquid surface depression will inevitably appear. The applied gas will cause a depression on the liquid surface, which will undoubtedly affect the plasma generation and further affect the application performance. However, the effect of liquid surface deformation on the plasma is still unclear. In this study, numerical models are developed to reveal the mechanism of liquid surface depressions affecting plasma discharge characteristics and the consequential distribution of plasma species, and further study the influence of liquid surface depressions of different sizes generated by different helium flow rates on the plasma. Results show that the liquid surface deformation changes the initial spatial electric field, resulting in the rearrangement of electrons on the liquid surface. The charges deposited on the liquid surface further increase the degree of distortion of the electric field. Moreover, the electric field and electron distribution affected by the liquid surface depression significantly influence the generation and distribution of active species, which determines the practical effectiveness of the relevant applications. This work explores the phenomenon of liquid surface depression, which has been neglected in previous related work, and contributes to further understanding of plasma-liquid interactions, providing better theoretical guidance for related applications and technologies.
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