西非城市阿比让(科特迪瓦)和阿克拉(加纳)PM2.5 的时间变化和区域影响†。

IF 2.8 Q3 ENVIRONMENTAL SCIENCES Environmental science: atmospheres Pub Date : 2024-03-19 DOI:10.1039/D4EA00012A
Julien Bahino, Michael Giordano, Matthias Beekmann, Véronique Yoboué, Arsène Ochou, Corinne Galy-Lacaux, Cathy Liousse, Allison Hughes, James Nimo, Farouk Lemmouchi, Juan Cuesta, A. Kofi Amegah and R. Subramanian
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引用次数: 0

摘要

微粒物质(PM)低成本传感器(LCS)可用于监测参考监测点有限地区的空气质量。在改善西非空气质量(IAQWA)项目框架内开展的这项研究,通过在阿比让(科特迪瓦)和阿克拉(加纳)部署经过现场校准的实时可负担多污染物(RAMP)监测器,提供了高时间分辨率的细气溶胶(PM2.5)质量浓度数据。2020 年 2 月至 2021 年 6 月,在阿比让的五个地点和阿克拉的四个地点部署了 RAMP。利用 15 秒的时间分辨率,RAMPs 提供的数据集可对不同污染源城市地点 PM2.5 浓度的日变化、日变化和季节变化进行长期比较分析。PM2.5 浓度的昼夜变化显示,与交通高峰期有关的早晨峰值明显,最高可达 50 μg m-3。傍晚的峰值在居民区的地点非常明显,并指向居民区类型的污染源。以年为周期对季节性差异进行分析,发现最大值出现在 12 月至次年 2 月的所谓长旱季(哈马丹)。在地面网络观测到的 2021 年 1 月的一次严重污染期间,三维卫星数据分析显示撒哈拉沙尘迁移是(细)气溶胶污染的额外来源,显著增加了 PM2.5。同一事件也揭示了 LCS 的局限性--无法充分捕捉以沙尘为主的污染,而这可以通过参考监测仪进行量化。年平均 PM2.5 浓度在 17 到 26 μg m-3 之间。城市内不同地点之间的 PM2.5 差异,尤其是受交通影响地点和城市背景地点之间的差异,要大于两个城市之间的差异。这些年平均值超过了世界卫生组织(WHO)2005 年(10 μg m-3)和 2021 年(5 μg m-3)指南的年污染阈值。
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Temporal variability and regional influences of PM2.5 in the West African cities of Abidjan (Côte d'Ivoire) and Accra (Ghana)†

Particulate Matter (PM) Low-Cost Sensors (LCS) can be used to monitor air quality in regions with limited access to reference monitors. This study carried out within the framework of the Improving Air Quality in West Africa (IAQWA) project provides high temporal resolution of data on fine aerosol (PM2.5) mass concentrations in Abidjan (Cote d'Ivoire) and Accra (Ghana) through the deployment of field calibrated Real-time Affordable Multi-pollutant (RAMP) monitors. From February 2020 to June 2021, RAMPs were deployed at five sites in Abidjan and four sites in Accra. Using a temporal resolution of 15 seconds, the datasets provided by RAMPs allowed a comparative analysis of diurnal, daily and seasonal variability of PM2.5 concentrations for different urban sites with distinct pollution sources, over an extended period of time. Diurnal variations in PM2.5 concentrations showed prominent morning peaks related to traffic rush hours reaching up to 50 μg m−3. Evening peaks were significant for sites in residential neighborhoods, and pointed to residential type pollution sources. Seasonal differences are analysed over a yearly cycle and maximum values are found during the so-called long dry season (Harmattan), between December and February. During a prominent pollution episode in January 2021 observed by the ground network, analysis of 3D satellite data, revealed Saharan dust transport as an additional source of (fine) aerosol pollution significantly increasing PM2.5. The same episode also revealed a limitation of LCS – an inability to adequately capture dust-dominated pollution, which can be quantified by reference monitors. Annual average PM2.5 concentrations vary between 17 and 26 μg m−3. PM2.5 differences between sites within a city, especially between traffic impacted and urban background sites, are larger than the differences between the two cities. These annual averages exceed World Health Organization (WHO) annual pollution thresholds from the 2005 (10 μg m−3) and 2021 (5 μg m−3) guidelines.

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