哑铃形硅纳米块中超腔模式和磁共振产生的增强型二次谐波

Yuwei Yuan, Yunbao Zheng, Ouyang Min, Haihua Fan, Qiaofeng Dai, Haiying Liu, Li-Jun Wu
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摘要

适当尺寸的介电纳米结构可以激发电磁多极共振,从而有效促进光与物质的相互作用。光与纳米结构之间的相互作用能够增强近场的电磁场,从而改善纳米结构的非线性效应。我们展示了单个哑铃形硅纳米块(DS-SiNB)激活的超空腔模式和磁偶极子共振,从而捕获近场电磁场能量。通过利用纳米结构表面的局部电磁场,增强了二次谐波的产生。数值模拟显示,通过不断调整纳米块的长宽比 Lout/Ly(外边缘长度与 DS-SiNB 长度之比),磁四极(MQ)和全电偶极子(TED)可以耦合到同一辐射通道。当长宽比 Lout/Ly = 1 时,由 MQ 和 TED 干涉形成的超空腔模式在 λ1 = 1124 nm 处被激发。此外,由两个同方向磁偶极子(MD)耦合形成的强磁共振模式也在λ2 = 1124 nm处被激发。超空腔模式和强磁偶极子共振能有效捕捉纳米结构表面的电磁场,从而实现增强的二次谐波发生(SHG)。我们的研究提出了一种增强单个硅纳米结构非线性光学效应的新方法,这将有助于开发更高效的非线性光学器件。
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Enhanced second harmonic generation from supercavity mode and magnetic resonance in dumbbell-shaped silicon nanoblock
Electromagnetic multipole resonance can be excited by dielectric nanostructures of appropriate size to effectively promote light-matter interaction. The interactions between light and nanostructures have the capability to enhance the electromagnetic field in the near field, thereby improving the nonlinear effect of nanostructures. We illustrate that the supercavity mode and magnetic dipole resonance are activated by a single dumbbell-shaped silicon nanoblock (DS-SiNB), to trap the near-field electromagnetic field energy. Enhanced second harmonic generation is achieved by exploiting the localized electromagnetic field at the surface of the nanostructure. Numerical simulations reveal that magnetic quadrupole (MQ) and total electric dipole (TED) can be coupled to the same radiation channel by adjusting continuously the aspect ratio Lout/Ly (the outer edge length to the length of DS-SiNB) of the nanoblock. When the aspect ratio Lout/Ly = 1, the supercavity mode formed by the interference of MQ and TED is excited at λ1 = 1124 nm. And, the strong magnetic resonance mode formed by the coupling of two magnetic dipoles (MD) in the same direction is also excited at λ2 = 1124 nm. Supercavity mode and strong magnetic dipole resonance can effectively capture electromagnetic fields on the surface of nanostructures to attain enhanced second harmonic generation (SHG). Our study presents a novel approach to enhance the nonlinear optical effect of a single silicon nanostructure, which can lead to the development of more efficient nonlinear optical devices.
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