土壤风化增强导致二氧化碳减少的直接证据

IF 3.4 1区 地球科学 Q1 GEOCHEMISTRY & GEOPHYSICS Geochemical Perspectives Letters Pub Date : 2024-04-30 DOI:10.7185/geochemlet.2415
T. Linke, E.H. Oelkers, S.C. Möckel, S.R. Gislason
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引用次数: 0

摘要

由于发生在土壤中的过程很多,而且当前项目的时间跨度较短,因此要证明工程强化风化对大气二氧化碳的影响能力一直是个挑战。在此,我们报告了冰岛 Histic/Gleyic Andosol 中的碳平衡情况,该土壤在 3300 年间接受了大量的玄武岩尘埃,为量化强化风化作用的速率和长期后果提供了机会。添加的玄武岩尘埃自沉积以来持续溶解。土壤水的碱度比没有玄武岩尘埃的同等土壤高出 10 倍以上。考虑到土壤水暴露在大气中时的氧化和脱气作用,每年因碱度生成而减少的二氧化碳量为 0.17 吨 C ha-1 yr-1。这项研究验证了向土壤中添加细粒黑云母矿物的能力,即通过碱度输出来减缓大气中二氧化碳的增加。不过,土壤有机碳储量的诱导变化很可能主导了风化作用增强所产生的二氧化碳净减少量。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Direct evidence of CO2 drawdown through enhanced weathering in soils
The ability of engineered enhanced weathering to impact atmospheric CO2 has been challenging to demonstrate due to the many processes occurring in soils and the short time span of current projects. Here we report the carbon balance in an Icelandic Histic/Gleyic Andosol that has received large quantities of basaltic dust over 3300 years, providing opportunity to quantify the rates and long term consequences of enhanced weathering. The added basaltic dust has dissolved continuously since its deposition. The alkalinity of the soil waters is more than 10 times higher than in equivalent basalt dust-free soils. After accounting for oxidation and degassing when the soil waters are exposed to the atmosphere, the annual CO2 drawdown due to alkalinity generation is 0.17 t C ha−1 yr−1. This study validates the ability of fine grained mafic mineral addition to soils to attenuate increasing atmospheric CO2 by alkalinity export. Induced changes in soil organic carbon storage, however, likely dominate the net CO2 drawdown of enhanced weathering efforts.
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来源期刊
Geochemical Perspectives Letters
Geochemical Perspectives Letters Earth and Planetary Sciences-Geochemistry and Petrology
CiteScore
7.00
自引率
2.00%
发文量
42
审稿时长
15 weeks
期刊介绍: Geochemical Perspectives Letters is an open access, internationally peer-reviewed journal of the European Association of Geochemistry (EAG) that publishes short, highest-quality articles spanning geochemical sciences. The journal aims at rapid publication of the most novel research in geochemistry with a focus on outstanding quality, international importance, originality, and stimulating new developments across the vast array of geochemical disciplines.
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