二维锗/锰离子范德华异质结构中的本征谷极化量子反常霍尔效应

Xiao-jing Dong, Chang-Wen Zhang
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摘要

谷极化量子反常霍尔效应(VQAHE)结合了非难带拓扑学和谷电学,对基础科学和新兴应用都具有重要意义。然而,这一特性的实验实现却面临挑战。在此,我们通过第一原理计算和模态分析,预测了在二维铁磁范德华锗/MnI2 异质结构中产生 VQAHE 的机制。在反常霍尔电导和手性边缘状态的帮助下,由于磁交换效应和自旋轨道耦合的共同作用,这种异质结构同时表现出山谷反常霍尔效应和 VQAHE。此外,有趣的是,通过对 In2Se3 中铁电极化态的电调制,锗/锰离子/In2Se3 异质结构可以实现从半导体到金属行为的可逆转换。这项工作为在铁磁范德华异质结构中寻找 VQAHE 以及利用基于 VQAHE 的高能效器件提供了指导性进展。
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Intrinsic valley-polarized quantum anomalous Hall effect in a two-dimensional germanene/MnI2 van der Waals heterostructure
Valley-polarized quantum anomalous Hall effect (VQAHE), combined nontrivial band topology with valleytronics, is of importance for both fundamental sciences and emerging applications. However, the experimental realization of this property is challengeable. Here, by using first-principles calculations and modal analysis, we predict a mechanism of producing VQAHE in two-dimensional ferromagnetic van der Waals germanene/MnI2 heterostructure. This heterostructure exhibits both valley anomalous Hall effect and VQAHE due to the joint effects of magnetic exchange effect and spin-orbital coupling with the aid of anomalous Hall conductance and chiral edge state. Moreover interestingly, through the electrical modulation of ferroelectric polarization state in In2Se3, the germanene/MnI2/In2Se3 heterostructure can undergo reversible switching from a semiconductor to a metallic behavior. This work offers a guiding advancement for searching for VQAHE in ferromagnetic van der Waals heterostructures and exploiting energy-efficient devices based on the VQAHE.
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