Yaxu Sun , Zhihan Tong , Yanyan Yu , Wanke Cheng , Yilin Li , Suqing Zeng , Yuhan Lou , Yongzhuang Liu , Qinqin Xia , Haipeng Yu
{"title":"溶剂对碳水化合物转化的影响：对化学途径调节的见解","authors":"Yaxu Sun , Zhihan Tong , Yanyan Yu , Wanke Cheng , Yilin Li , Suqing Zeng , Yuhan Lou , Yongzhuang Liu , Qinqin Xia , Haipeng Yu","doi":"10.1039/d3gc04901a","DOIUrl":null,"url":null,"abstract":"<div><p>Carbohydrate utilization is a crucial aspect of sustainable resource development and offers a promising avenue for replacing fossil fuels. In carbohydrate reaction systems, solvent effects influence the interactions among carbohydrates, catalysts, and solvents. These can affect the reaction trajectory and selectivity, making them a crucial tool for cost-effectively regulating reactions. This review summarizes the primary types of carbohydrate chemical transformation and commonly used solvent systems, providing an overview of solvent effects in these reactions and an insight into solvent effects from a microscopic perspective. Additionally, it provides insights into the current state of solvent engineering and the challenges limiting the development of solvent-based carbohydrate transformation systems.</p></div>","PeriodicalId":78,"journal":{"name":"Green Chemistry","volume":"26 12","pages":"Pages 6900-6925"},"PeriodicalIF":9.3000,"publicationDate":"2024-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Solvent effects on carbohydrate transformation: insights into chemical pathway modulation\",\"authors\":\"Yaxu Sun , Zhihan Tong , Yanyan Yu , Wanke Cheng , Yilin Li , Suqing Zeng , Yuhan Lou , Yongzhuang Liu , Qinqin Xia , Haipeng Yu\",\"doi\":\"10.1039/d3gc04901a\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Carbohydrate utilization is a crucial aspect of sustainable resource development and offers a promising avenue for replacing fossil fuels. In carbohydrate reaction systems, solvent effects influence the interactions among carbohydrates, catalysts, and solvents. These can affect the reaction trajectory and selectivity, making them a crucial tool for cost-effectively regulating reactions. This review summarizes the primary types of carbohydrate chemical transformation and commonly used solvent systems, providing an overview of solvent effects in these reactions and an insight into solvent effects from a microscopic perspective. Additionally, it provides insights into the current state of solvent engineering and the challenges limiting the development of solvent-based carbohydrate transformation systems.</p></div>\",\"PeriodicalId\":78,\"journal\":{\"name\":\"Green Chemistry\",\"volume\":\"26 12\",\"pages\":\"Pages 6900-6925\"},\"PeriodicalIF\":9.3000,\"publicationDate\":\"2024-06-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Green Chemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/org/science/article/pii/S1463926224005600\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Green Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/org/science/article/pii/S1463926224005600","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Solvent effects on carbohydrate transformation: insights into chemical pathway modulation
Carbohydrate utilization is a crucial aspect of sustainable resource development and offers a promising avenue for replacing fossil fuels. In carbohydrate reaction systems, solvent effects influence the interactions among carbohydrates, catalysts, and solvents. These can affect the reaction trajectory and selectivity, making them a crucial tool for cost-effectively regulating reactions. This review summarizes the primary types of carbohydrate chemical transformation and commonly used solvent systems, providing an overview of solvent effects in these reactions and an insight into solvent effects from a microscopic perspective. Additionally, it provides insights into the current state of solvent engineering and the challenges limiting the development of solvent-based carbohydrate transformation systems.
期刊介绍：
Green Chemistry is a journal that provides a unique forum for the publication of innovative research on the development of alternative green and sustainable technologies. The scope of Green Chemistry is based on the definition proposed by Anastas and Warner (Green Chemistry: Theory and Practice, P T Anastas and J C Warner, Oxford University Press, Oxford, 1998), which defines green chemistry as the utilisation of a set of principles that reduces or eliminates the use or generation of hazardous substances in the design, manufacture and application of chemical products. Green Chemistry aims to reduce the environmental impact of the chemical enterprise by developing a technology base that is inherently non-toxic to living things and the environment. The journal welcomes submissions on all aspects of research relating to this endeavor and publishes original and significant cutting-edge research that is likely to be of wide general appeal. For a work to be published, it must present a significant advance in green chemistry, including a comparison with existing methods and a demonstration of advantages over those methods.
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