评估硫化锌异质结构作为将二氧化碳转化为有价值化学品和清洁能源的催化剂的效果

IF 3.2 Q2 CHEMISTRY, PHYSICAL Energy advances Pub Date : 2024-05-23 DOI:10.1039/D4YA00202D
Onome Ejeromedoghene, Khadijat Olabisi Abdulwahab, Inemesit Asukwo Udofia, Moses Kumi and Ayorinde Olufunke Nejo
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摘要

由于大气中二氧化碳(CO2)浓度的上升和化石燃料的枯竭,全球变暖和能源危机备受关注。利用丰富的太阳能将二氧化碳转化为有机分子将是解决这两个问题的快速方法。过量的二氧化碳是导致全球变暖、极端天气模式和其他一系列环境挑战的温室效应的主要因素。为了解决这些问题,科学家们正在探索吸附二氧化碳的新方法,将其转化为有用的产品,然后再释放回大气中。半导体材料在二氧化碳还原过程中发挥着至关重要的作用。在这些材料中,硫化锌(ZnS)和掺杂 ZnS 因可能催化二氧化碳转化为有用化合物而备受关注。ZnS 及其衍生物的半导体特性使其特别适合于这一目的。本综述概述了在开发具有二氧化碳还原功能特性的 ZnS 基异质结构方面的最新进展。本综述还探讨了二氧化碳的转化机制,并对计算建模提出了新的见解。最后,还对用于还原二氧化碳的 ZnS 基催化材料的未来发展进行了展望。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Evaluation of zinc sulfide heterostructures as catalysts for the transformation of CO2 into valuable chemicals and clean energy generation

There are significant concerns about global warming and the energy crisis due to the rise in atmospheric carbon dioxide (CO2) concentration and the depletion of fossil fuels. Converting CO2 into organic molecules using the abundant solar energy would be a quick fix that would address both issues. Excess CO2 is a major contributor to the greenhouse effect, which leads to global warming, extreme weather patterns, and a host of other environmental challenges. To tackle these problems, scientists are exploring novel approaches to adsorb CO2, transform it into useful products, and then release it back into the atmosphere. Semiconductor materials play a crucial role in CO2 reduction. Among these materials, zinc sulfide (ZnS) and doped ZnS have gained significant attention for the potential catalytic transformation of CO2 into useful compounds. The semiconductor properties of ZnS and its derivatives make them particularly well-suited for this purpose. The present review provides a summary of the recent progress in the development of strategies for fabricating ZnS-based heterostructures with functional properties for CO2 reduction. The mechanism of CO2 conversion was also addressed with new insights into computational modelling. Lastly, future outlook on the development of catalytic ZnS-based materials for CO2 reduction is provided.

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Correction: Steady states and kinetic modelling of the acid-catalysed ethanolysis of glucose, cellulose, and corn cob to ethyl levulinate. Back cover Fabrication methods, pseudocapacitance characteristics, and integration of conjugated conducting polymers in electrochemical energy storage devices Inside back cover Back cover
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