具有朗缪尔型吸附作用的体表反应-吸附-扩散系统分析

IF 4.6 Q2 MATERIALS SCIENCE, BIOMATERIALS ACS Applied Bio Materials Pub Date : 2024-05-28 DOI:10.1016/j.matpur.2024.05.001
Björn Augner, Dieter Bothe
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引用次数: 0

摘要

我们考虑一类体相-表面反应-吸附-扩散系统,即有界域Ω⊆Rd(体相)及其边界Σ=∂Ω(表面相)上的反应-扩散耦合系统,它们通过非线性法向通量边界条件耦合。特别是,这类模型包括一个异相催化模型,它具有费克式的体相和表面扩散以及朗缪尔式的非线性吸附,即从体相到活性表面的传输和解吸。对于这个模型,我们在化学反应网络和吸附模型的一些现实结构条件下,获得了求解的好求解性、正求解性和全局时间存在性。我们在适当的 Sobolev-Slobodetskii 设置下进行研究,我们的目标是在较宽的范围内获得可积分性指数,包括特定值 p<d。
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Analysis of bulk-surface reaction-sorption-diffusion systems with Langmuir-type adsorption

We consider a class of bulk-surface reaction-adsorption-diffusion systems, i.e. a coupled system of reaction-diffusion systems on a bounded domain ΩRd (bulk phase) and its boundary Σ=Ω (surface phase), which are coupled via nonlinear normal flux boundary conditions. In particular, this class includes a heterogeneous catalysis model with Fickian bulk and surface diffusion and nonlinear adsorption of Langmuir type, i.e. transport from the bulk phase to the active surface, and desorption. For this model, we obtain well-posedness, positivity and global-in-time existence of solutions under some realistic structural conditions on the chemical reaction network and the sorption model. We work in appropriate Sobolev-Slobodetskii settings, where we aim for a wide range for the integrability index, including in particular values p<d.

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来源期刊
ACS Applied Bio Materials
ACS Applied Bio Materials Chemistry-Chemistry (all)
CiteScore
9.40
自引率
2.10%
发文量
464
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