由相变量子点弦固有非线性演变而来的自适应信号调制。

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2024-06-20 DOI:10.1021/acs.nanolett.4c01786
Qin Wan, Fei Zeng*, Ziao Lu, Junwei Yu, Tongjin Chen and Feng Pan, 
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引用次数: 0

摘要

要通过随机共振(SR)模拟处理微弱信号的拓扑神经网络,就必须在纳米级器件中引入固有的非线性。我们利用自组装方法成功地制造出了跨越 Pd/Nb:AlNO/AlNO/Nb:AlNO/Pd 多层的相变量子点串(PCQDS)。相变的固有非线性与电子隧道耦合,使 PCQDS 能够以调制输出方式响应长信号序列,其中脉冲模式演变为由两组周期性波包围的神经动作电位模式。我们建立了一种由多个双态系统组成的 SR 模式,其中耗散隧道与环境耦合。NbO QD 的尺寸振荡会自适应地调整壁垒和阱,从而使隧穿受到非对称能量或局部温度的周期性调制。当施加外部周期性信号时,系统首先跟随强迫频率。随后,某些 PCQD 独立并连续振荡,产生复杂的频率和振幅调制。
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Adaptive Signal Modulation Evolved by the Inherent Nonlinearity of Phase-Change Quantum-Dot String

To simulate a topological neural network handling weak signals via stochastic resonance (SR), it is necessary to introduce an inherent nonlinearity into nanoscale devices. We use the self-assembly method to successfully fabricate a phase-change quantum-dot string (PCQDS) crossing Pd/Nb:AlNO/AlNO/Nb:AlNO/Pd multilayer. The inherent nonlinearity of phase change couples with electron tunneling so that PCQDS responds to a long signal sequence in a modulated output style, in which the pulse pattern evolves to that enveloped by two sets of periodic wave characterized by neural action potential. We establish an SR mode consisting of several two-state systems in which dissipative tunneling is coupled to environment. Size oscillations owing to NbO QDs adaptively adjust barriers and wells, such that tunneling can be periodically modulated by either asymmetric energy or local temperature. When the external periodic signals are applied, the system first follows the forcing frequency. Subsequently, certain PCQDs oscillate independently and consecutively to produce complicated frequency and amplitude modulations.

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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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