{"title":"基于具有环状偶极子共振的浮动双层元表面的太赫兹传感技术实现超高灵敏度","authors":"Xiaoxuan Liu, Binggang Xiao, Jianyuan Qin","doi":"10.1002/adom.202400785","DOIUrl":null,"url":null,"abstract":"<p>Metasurface structures have proven to be effective in enhancing terahertz sensing signals and can thus be used as sensors to improve terahertz detection sensitivity. However, the sensitivity is limited by the poor spatial overlap between the analytes and the local electric field of the metasurface. In this work, a novel design of a floating bilayer metasurface structure for terahertz sensing is proposed and investigated. This structure supports a sharp toroidal dipole resonance and can concentrate near-field energy on the analyte and metal atoms rather than on the substrate surface by floating the metal atoms. Consequently, the sensitivity is significantly improved to as high as 362 GHz RIU<sup>−1</sup>; theoretically, this is approximately 2.6 times higher than that of the common metasurface. The ability of the floating bilayer metasurface to quantitatively detect chlorothalonil is experimentally demonstrated. The resonance peak shows a significant frequency shift of 7 GHz for a change of 0.0001 mg dL<sup>−1</sup> in chlorothalonil concentration, reaching up to 86 GHz when the change in chlorothalonil concentration is 100 mg dL<sup>−1</sup>; this is approximately 6.6 times higher than that of the common metasurface. This work provides opportunities for metasurface to realize ultrasensitive sensing in the terahertz regime.</p>","PeriodicalId":116,"journal":{"name":"Advanced Optical Materials","volume":null,"pages":null},"PeriodicalIF":8.0000,"publicationDate":"2024-07-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Terahertz Sensing Based on Floating Bilayer Metasurface with Toroidal Dipole Resonance Toward Ultra-High Sensitivity\",\"authors\":\"Xiaoxuan Liu, Binggang Xiao, Jianyuan Qin\",\"doi\":\"10.1002/adom.202400785\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Metasurface structures have proven to be effective in enhancing terahertz sensing signals and can thus be used as sensors to improve terahertz detection sensitivity. However, the sensitivity is limited by the poor spatial overlap between the analytes and the local electric field of the metasurface. In this work, a novel design of a floating bilayer metasurface structure for terahertz sensing is proposed and investigated. This structure supports a sharp toroidal dipole resonance and can concentrate near-field energy on the analyte and metal atoms rather than on the substrate surface by floating the metal atoms. Consequently, the sensitivity is significantly improved to as high as 362 GHz RIU<sup>−1</sup>; theoretically, this is approximately 2.6 times higher than that of the common metasurface. The ability of the floating bilayer metasurface to quantitatively detect chlorothalonil is experimentally demonstrated. The resonance peak shows a significant frequency shift of 7 GHz for a change of 0.0001 mg dL<sup>−1</sup> in chlorothalonil concentration, reaching up to 86 GHz when the change in chlorothalonil concentration is 100 mg dL<sup>−1</sup>; this is approximately 6.6 times higher than that of the common metasurface. This work provides opportunities for metasurface to realize ultrasensitive sensing in the terahertz regime.</p>\",\"PeriodicalId\":116,\"journal\":{\"name\":\"Advanced Optical Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":8.0000,\"publicationDate\":\"2024-07-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Optical Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/adom.202400785\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Optical Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/adom.202400785","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Terahertz Sensing Based on Floating Bilayer Metasurface with Toroidal Dipole Resonance Toward Ultra-High Sensitivity
Metasurface structures have proven to be effective in enhancing terahertz sensing signals and can thus be used as sensors to improve terahertz detection sensitivity. However, the sensitivity is limited by the poor spatial overlap between the analytes and the local electric field of the metasurface. In this work, a novel design of a floating bilayer metasurface structure for terahertz sensing is proposed and investigated. This structure supports a sharp toroidal dipole resonance and can concentrate near-field energy on the analyte and metal atoms rather than on the substrate surface by floating the metal atoms. Consequently, the sensitivity is significantly improved to as high as 362 GHz RIU−1; theoretically, this is approximately 2.6 times higher than that of the common metasurface. The ability of the floating bilayer metasurface to quantitatively detect chlorothalonil is experimentally demonstrated. The resonance peak shows a significant frequency shift of 7 GHz for a change of 0.0001 mg dL−1 in chlorothalonil concentration, reaching up to 86 GHz when the change in chlorothalonil concentration is 100 mg dL−1; this is approximately 6.6 times higher than that of the common metasurface. This work provides opportunities for metasurface to realize ultrasensitive sensing in the terahertz regime.
期刊介绍:
Advanced Optical Materials, part of the esteemed Advanced portfolio, is a unique materials science journal concentrating on all facets of light-matter interactions. For over a decade, it has been the preferred optical materials journal for significant discoveries in photonics, plasmonics, metamaterials, and more. The Advanced portfolio from Wiley is a collection of globally respected, high-impact journals that disseminate the best science from established and emerging researchers, aiding them in fulfilling their mission and amplifying the reach of their scientific discoveries.