单层半导体中激子振荡器强度和空间分布的电气控制

IF 9.5 2区 材料科学 Q1 CHEMISTRY, PHYSICAL Nano Research Pub Date : 2024-07-01 DOI:10.1007/s12274-024-6762-7
Yanming Wang, Junrong Zhang, Tianhua Ren, Meng Xia, Long Fang, Xiangyi Wang, Xingwang Zhang, Kai Zhang, Junyong Wang
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引用次数: 0

摘要

发光的电调制对现代发光设备意义重大。单层过渡金属二掺镓化合物是新兴的直带隙发光材料,具有独特的激子特性,多种激子复合物为调制原子级薄半导体的发光特性提供了新的机会。在这里,我们报告了在单层 WS2 中对激子发射的振荡器强度和空间分布的电学控制。在室温下,通过电场对激子发射强度进行了有效调制,调制度达到约 92%。通过横向电场调整空间载流子再分布,可以设计出不同的激子发射模式。激子振荡器强度和分布的调制方法为研究激子扩散动力学和构建电可调光电器件提供了有效途径。
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Electrical control of excitonic oscillator strength and spatial distribution in a monolayer semiconductor

Electrical modulation of luminescence is significant to modern light-emitting devices. Monolayer transition metal dichalcogenides are emerging direct-bandgap luminescent materials with unique excitonic properties, and the multiple exciton complexes provide new opportunities to modulate the property of luminescence in atomically thin semiconductors. Here, we report an electrical control of exciton emission in the oscillator strength and spatial distribution of excitons in a monolayer WS2. Effective modulation of excitonic emission intensity with a degree of modulation of ~ 92% has been demonstrated by an electric field at room temperature. The spatial carrier redistribution tuned by a lateral electric field results in distinct excitonic emission patterns by design. The modulation approach to exciton oscillator strength and distribution provides an efficient way to investigate the exciton diffusion dynamics and to construct electrically tunable optoelectronic devices.

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来源期刊
Nano Research
Nano Research 化学-材料科学:综合
CiteScore
14.30
自引率
11.10%
发文量
2574
审稿时长
1.7 months
期刊介绍: Nano Research is a peer-reviewed, international and interdisciplinary research journal that focuses on all aspects of nanoscience and nanotechnology. It solicits submissions in various topical areas, from basic aspects of nanoscale materials to practical applications. The journal publishes articles on synthesis, characterization, and manipulation of nanomaterials; nanoscale physics, electrical transport, and quantum physics; scanning probe microscopy and spectroscopy; nanofluidics; nanosensors; nanoelectronics and molecular electronics; nano-optics, nano-optoelectronics, and nano-photonics; nanomagnetics; nanobiotechnology and nanomedicine; and nanoscale modeling and simulations. Nano Research offers readers a combination of authoritative and comprehensive Reviews, original cutting-edge research in Communication and Full Paper formats. The journal also prioritizes rapid review to ensure prompt publication.
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