Shi Wang, Shijun Xiao, Henan Cai, Wenqing Sun, Tong Wu, Yu Wang, Jixin He, Sheng Yang, Zhen-Dong Huang, Wen-Yong Lai
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Elastic Polymer Electrolytes Integrated with In Situ Polymerization-Transferred Electrodes toward Stretchable Batteries
Stretchable Li-ion batteries (LIBs) are important potential power sources for flexible electronics. Here, we propose an integrated in situ polymerization-transfer strategy to construct intrinsically stretchable LIBs (is-LIBs). Specifically, a polymer electrolyte (PE) with chain-liquid synergistic effect by poly(ethylene glycol methyl ether acrylate)-ionic liquid/lithium salt has been developed, which facilitates rapid Li+ transport (10–4 S cm–1) and promotes mechanical flexibility (stretching over 5000%) due to the unique phase-separated structure of the PE and the ionic–bipolar interactions between the C=O-rich polymer and imidazolium cations. Additionally, Ag nanowires (AgNWs)/electrode materials are transferred to PDMS to construct intrinsically stretchable electrodes. The strong physical interaction between AgNWs/electrode materials and PDMS endows electrodes with a high strain of 100% and low sheet resistance of 0.9 Ω □–1. Finally, an is-LIB is achieved by in situ polymerization-transfer integration, showing good cycle and rate performance. The results suggest a new avenue for the development of stretchable energy storage devices.
ACS Energy Letters Energy-Renewable Energy, Sustainability and the Environment
CiteScore
31.20
自引率
5.00%
发文量
469
审稿时长
1 months
期刊介绍:
ACS Energy Letters is a monthly journal that publishes papers reporting new scientific advances in energy research. The journal focuses on topics that are of interest to scientists working in the fundamental and applied sciences. Rapid publication is a central criterion for acceptance, and the journal is known for its quick publication times, with an average of 4-6 weeks from submission to web publication in As Soon As Publishable format.
ACS Energy Letters is ranked as the number one journal in the Web of Science Electrochemistry category. It also ranks within the top 10 journals for Physical Chemistry, Energy & Fuels, and Nanoscience & Nanotechnology.
The journal offers several types of articles, including Letters, Energy Express, Perspectives, Reviews, Editorials, Viewpoints and Energy Focus. Additionally, authors have the option to submit videos that summarize or support the information presented in a Perspective or Review article, which can be highlighted on the journal's website. ACS Energy Letters is abstracted and indexed in Chemical Abstracts Service/SciFinder, EBSCO-summon, PubMed, Web of Science, Scopus and Portico.