[基于 XGBoost-LME 模型的京津冀地区近地面臭氧浓度估算]。

Q2 Environmental Science Huanjing Kexue/Environmental Science Pub Date : 2024-07-08 DOI:10.13227/j.hjkx.202307110
De-Cai Gong, Ning Du, Li Wang, Xian-Yun Zhang, Long Li, Hong-Fei Zhang
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引用次数: 0

摘要

近地面臭氧浓度分布的高时空分辨率数据对于监测和控制大气臭氧污染、改善生活环境具有重要意义。利用 TROPOMI-L3 NO2、HCHO 产物和 ERA5-陆地高分辨率数据作为估算变量,构建了 XGBoost-LME 模型,对京津冀地区近地面臭氧浓度进行了估算。对流层甲醛(HCHO)和对流层二氧化氮(NO2)。是影响京津冀地区近地面臭氧浓度的重要因素。其中,T2M、SSRD 和 D2M 的相关性较强,相关系数分别为 0.82、0.75 和 0.71。与其他模型相比,XGBoost-LME 模型的各项指标表现最好。十倍交叉验证评价指标 R2、MAE 和 RMSE 分别为 0.951、9.27 μg-m-3 和 13.49 μg-m-3。同时,该模型在不同时间尺度下均表现良好。从时间上看,2019 年京津冀地区近地面臭氧浓度存在明显的季节性差异,浓度变化顺序依次为夏季> 春季> 秋季> 冬季。全区臭氧月平均浓度呈倒 "V "型变化趋势,9 月份略有上升。最高值出现在 7 月,最低值出现在 12 月。从空间分布来看,京津冀地区 2 月和 3 月的近地面臭氧浓度基本处于同一水平。在 1 月、11 月和 12 月,北部浓度较高,南部浓度较低的趋势相对不明显。在其余月份,该地区近地面臭氧浓度的空间分布主要呈现出南部浓度较高,北部浓度较低的模式。高值区主要分布在南部的平原地区,海拔较低、人口密集、工业排放量较高;而低值区主要分布在北部的山区,海拔较高、人口稀少、植被覆盖率较高、工业排放量较低。
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[Estimation of Near-surface Ozone Concentration in the Beijing-Tianjin-Hebei Region Based on XGBoost-LME Model].

High spatiotemporal resolution data on near-surface ozone concentration distribution is of great significance for monitoring and controlling atmospheric ozone pollution and improving the living environment. Using TROPOMI-L3 NO2, HCHO products, and ERA5-land high-resolution data as estimation variables, an XGBoost-LME model was constructed to estimate the near-surface ozone concentration in the Beijing-Tianjin-Hebei Region. The results showed that: ① Through correlation analysis, surface 2 m temperature (T2M), 2 m dewpoint temperature (D2M), surface solar radiation downwards (SSRD), tropospheric formaldehyde (HCHO), and tropospheric nitrogen dioxide (NO2) were important factors affecting the near-surface ozone concentration in the Beijing-Tianjin-Hebei Region. Among them, T2M, SSRD, and D2M had strong correlations, with correlation coefficients of 0.82, 0.75, and 0.71, respectively. ② Compared with that of other models, the XGBoost-LME model had the best performance in terms of various indicators. The ten-fold cross-validation evaluation indicators R2, MAE, and RMSE were 0.951, 9.27 μg·m-3, and 13.49 μg·m-3, respectively. At the same time, the model performed well at different time scales. ③ In terms of time, there was a significant seasonal difference in near-surface ozone concentration in the Beijing-Tianjin-Hebei Region in 2019, with the concentration changing in the order of summer > spring > autumn > winter. The monthly average ozone concentration in the region showed an inverted "V" trend, with a slight increase in September. The highest value occurred in July, whereas the lowest value occurred in December. In terms of spatial distribution, the near-surface ozone concentrations in the Beijing-Tianjin-Hebei Region during the months of February and March were generally at the same levels. In January, November, and December, there was a relatively insignificant trend of higher concentrations in the north and lower concentrations in the south. For the remaining months, the spatial distribution of near-surface ozone concentrations in this area predominantly exhibited a pattern of higher concentrations in the south and lower concentrations in the north. High-value areas were predominantly found in the plain regions of the southern part with lower altitudes, dense population, and higher industrial emissions; low-value areas, on the other hand, were primarily located in mountainous areas of the northern part with higher altitudes, sparse population, higher vegetation coverage, and lower industrial emissions.

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来源期刊
Huanjing Kexue/Environmental Science
Huanjing Kexue/Environmental Science Environmental Science-Environmental Science (all)
CiteScore
4.40
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15329
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