大气气溶胶对区域极端天气和气候事件的影响综述

IF 1.6 4区 环境科学与生态学 Q4 ENVIRONMENTAL SCIENCES Aerosol Science and Engineering Pub Date : 2024-07-15 DOI:10.1007/s41810-024-00223-x
Julius A. Akinyoola, A. Oluleye, Imoleayo E. Gbode
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引用次数: 0

摘要

大气气溶胶是大气的基本成分,也与辐射和云层相互作用。自工业时代以来,主要在观测、理解和模拟过程方面取得了重大进展,这些研究工作有助于确定气溶胶的光学特性如何对影响区域和全球气候的辐射强迫产生作用。研究结果还有助于量化人为气溶胶造成的地球辐射预算失衡,以及气溶胶在区域和全球范围内造成全球变暖的其他各种方式。目前已经开发了几种气溶胶清单来量化不同种类的气溶胶,包括排放、寿命、大小、从一个地区到另一个地区的运输,以及周围环境对气溶胶特性的影响。近来,为充分测量气溶胶辐射和云层相互作用,开发了新的指标,包括气溶胶瞬时辐射强迫(IRF),它是由于气溶胶与进入的太阳辐射或传出的红外辐射直接相互作用而导致的地球能量平衡变化,可导致大气变暖或变冷,具体取决于气溶胶类型(例如,硫酸盐气溶胶会导致变冷)。快速调整也指大气对辐射强迫变化的快速反应,包括温度、湿度和云量的调整。它几乎立即发生,与气溶胶或温室气体排放一起影响当地和区域气候条件。另一方面,在考虑了快速修正和反馈之后,有效辐射强迫(ERF)代表了地球能量平衡的净变化。通过记录短期和长期反馈,它可以更全面地了解气溶胶或其他物质对气候的总体影响。这些指标被用来精确估算净辐射扰动,尽管这三个新近开发的指标的实际测量值在各个地区仍有莫名的波动。本综述介绍了气溶胶特性的各个方面,特别是与辐射、云相互作用和极端事件有关的方面。向建模方法、理论考虑和微调观测方法的新范式转变是需要考虑的重要工具。气溶胶的散射和吸收显示了气溶胶与短波和长波辐射相互作用时所涉及的不同机制,但气溶胶的吸收能力可能并不像研究共识中所说的那样仅限于某些气溶胶种类,这些可能是气溶胶与辐射相互作用产生的地表辐射通量的主要制约因素之一。研究还考虑了人为气溶胶对云液态水含量和云分量的影响,发现这些复杂的过程不太清楚,对混合云和冰云的影响仍有待深入了解。由于辐射扰动以及大气顶部和地表的辐射通量,观测到的地表温度上升变化是全球变暖的主要驱动力,同时也对天气和气候极端事件产生影响。高精度测量地表温度的变化也非常重要。气溶胶是降水过程中水汽的主要载体,气溶胶引起的变暖对全球环流的影响程度还有待充分探讨。与洪水事件相关的极端事件以及与极端温度和热浪相关的干旱事件是当前和未来研究的关键领域。总之,与传统的直接和间接气溶胶辐射强迫相比,如果我们必须考虑准确和科学地量化所发明的三种指标的重要性和使用方法,那么就需要正确理解和采用更好的研究方法来消除对这方面不确定性的担忧。新技术工具的应用和新参数化方案的开发是需要考虑的重要因素,这些工具和方案可以表达气溶胶与气候之间的微观相互作用和过程,这些相互作用和过程规模较小,无法在区域和全球尺度上明确解决或捕捉。
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A Review of Atmospheric Aerosol Impacts on Regional Extreme Weather and Climate Events

Atmospheric aerosols are essential constituents of the atmosphere and also interact with radiation and clouds. Substantial progress has been made since the industrial era majorly for observing, understanding, and modeling processes and these research efforts have helped to identify how aerosol optical properties have contributed to radiative forcing that influence regional and global climate. Research findings have also helped to quantify the imbalance in the Earth's radiation budget caused by anthropogenic aerosols as well as various other ways aerosol has contributed to global warming both at the regional and global scale. Several aerosol inventories have been developed to quantify different aerosol species including the emission, life span, sizes, and transportation from one region to another and as well as the influence of the surrounding environment on aerosol characteristics. In recent times new metrics have been developed for adequate measurements to quantifying aerosol radiation and cloud interaction including Aerosol Instantaneous Radiative Forcing (IRF) which is the changes that occur in the Earth's energy balance due to the direct interaction of aerosols with incoming solar or outgoing infrared radiation and can lead to warming or cooling of the atmosphere, depending on the aerosol type (e.g., sulfate aerosols cause cooling). Rapid adjustment also referred to as a swift in atmospheric response to changes in radiative forcing, including adjustments in temperature, humidity, and cloud cover. It occurs almost immediately, influencing local and regional climate conditions alongside aerosol or greenhouse gas emissions. On the other hand, after taking into consideration quick corrections and feedbacks, the Effective Radiative Forcing (ERF) represents the net change in Earth's energy balance. By recording both short- and long-term feedbacks, it offers a more thorough knowledge of the total impact of aerosols or other agents on climate. These metrics are employed to precisely estimate net radiation perturbation, even though the actual measurement values of these three recently developed metrics continue to fluctuate inexplicably throughout the regions. This review provides information on various aspects of aerosol properties especially those that are related to radiation, cloud interaction, and extreme events. The new paradigm shifts to a modeling approach, theoretical considerations, and finetuned observational methodology are essential tools to be considered. Scattering and absorption of aerosol show different mechanisms involved when aerosols interact with short and long-wave radiation but aerosol absorption ability might not only be limited to certain aerosol species as entailed in research consensus and these might be one of the major constraints of surface radiative fluxes from aerosol-radiation interactions. The influence of anthropogenic aerosols on cloud liquid water content and cloud fraction was also considered and it has been discovered that these complex processes are less clear, and the influence on mixed-phase and ice clouds remains to be well understood. Observed changes in surface temperature increase due to radiation perturbation and the radiative fluxes both at the Top of the Atmosphere and at the surface are the major driving force for global warming and also impacts weather and climate extreme events. It is also very important to measure with high sense of accuracy the changes in the surface temperature. The degree of aerosol-induced warming on global circulation as the major carrier of moisture for precipitation processes is yet to be fully explored. The extreme events associated with flood events and as well as drought associated with extreme temperature and heat waves are key areas for current and future research. In summary, if we must consider importance and the usage of the three invented metrics for accurate and scientific quantification over the traditional Direct and Indirect aerosol radiative forcing then there is a need for proper understanding and a better research approach to allay the fear of uncertainty in this regard. The application of new technological tools and as well as new parametrization schemes development that express micro aerosol-climate interaction and processes that are smaller and cannot be resolved or captured explicitly on regional and global scales are important factors to be considered.

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来源期刊
Aerosol Science and Engineering
Aerosol Science and Engineering Environmental Science-Pollution
CiteScore
3.00
自引率
7.10%
发文量
42
期刊介绍: ASE is an international journal that publishes high-quality papers, communications, and discussion that advance aerosol science and engineering. Acceptable article forms include original research papers, review articles, letters, commentaries, news and views, research highlights, editorials, correspondence, and new-direction columns. ASE emphasizes the application of aerosol technology to both environmental and technical issues, and it provides a platform not only for basic research but also for industrial interests. We encourage scientists and researchers to submit papers that will advance our knowledge of aerosols and highlight new approaches for aerosol studies and new technologies for pollution control. ASE promotes cutting-edge studies of aerosol science and state-of-art instrumentation, but it is not limited to academic topics and instead aims to bridge the gap between basic science and industrial applications.  ASE accepts papers covering a broad range of aerosol-related topics, including aerosol physical and chemical properties, composition, formation, transport and deposition, numerical simulation of air pollution incidents, chemical processes in the atmosphere, aerosol control technologies and industrial applications. In addition, ASE welcomes papers involving new and advanced methods and technologies that focus on aerosol pollution, sampling and analysis, including the invention and development of instrumentation, nanoparticle formation, nano technology, indoor and outdoor air quality monitoring, air pollution control, and air pollution remediation and feasibility assessments.
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