{"title":"减轻氧还原反应障碍:高熵合金催化剂的深入第一原理探索","authors":"Ming-Yi Chen , Ngoc Thanh Thuy Tran , Wen-Dung Hsu","doi":"10.1016/j.elecom.2024.107782","DOIUrl":null,"url":null,"abstract":"<div><p>This study investigates the effectiveness of high-entropy alloys (HEAs) as catalysts for reducing the energy barrier of the oxygen reduction reaction (ORR) in proton exchange membrane fuel cells (PEMFCs). Four HEAs—IrPdPtRh, CoCrFeNi, NbMoTaW, and TiZrNbTa—are analyzed as potential catalysts. This superiority arises from the shift in the overall d-band center position towards negative energy in HEAs. The study suggests that an increased standard deviation of atomic valences within HEAs correlates positively with improved ORR efficiency, indicating it as a potential design indicator for cost-effective catalysts. Moreover, predictions of valence variations based on differences in electronegativity between individual elements are proposed. Additionally, the research highlights that additional surface adsorption of Pt on HEAs would further enhance ORR activity.</p></div>","PeriodicalId":304,"journal":{"name":"Electrochemistry Communications","volume":"166 ","pages":"Article 107782"},"PeriodicalIF":4.7000,"publicationDate":"2024-07-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S1388248124001255/pdfft?md5=248509447dc76ae79b535d41868a354a&pid=1-s2.0-S1388248124001255-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Mitigating oxygen reduction reaction barriers: An in-depth first-principles exploration of high-entropy alloy as catalysts\",\"authors\":\"Ming-Yi Chen , Ngoc Thanh Thuy Tran , Wen-Dung Hsu\",\"doi\":\"10.1016/j.elecom.2024.107782\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>This study investigates the effectiveness of high-entropy alloys (HEAs) as catalysts for reducing the energy barrier of the oxygen reduction reaction (ORR) in proton exchange membrane fuel cells (PEMFCs). Four HEAs—IrPdPtRh, CoCrFeNi, NbMoTaW, and TiZrNbTa—are analyzed as potential catalysts. This superiority arises from the shift in the overall d-band center position towards negative energy in HEAs. The study suggests that an increased standard deviation of atomic valences within HEAs correlates positively with improved ORR efficiency, indicating it as a potential design indicator for cost-effective catalysts. Moreover, predictions of valence variations based on differences in electronegativity between individual elements are proposed. Additionally, the research highlights that additional surface adsorption of Pt on HEAs would further enhance ORR activity.</p></div>\",\"PeriodicalId\":304,\"journal\":{\"name\":\"Electrochemistry Communications\",\"volume\":\"166 \",\"pages\":\"Article 107782\"},\"PeriodicalIF\":4.7000,\"publicationDate\":\"2024-07-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S1388248124001255/pdfft?md5=248509447dc76ae79b535d41868a354a&pid=1-s2.0-S1388248124001255-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Electrochemistry Communications\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1388248124001255\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ELECTROCHEMISTRY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Electrochemistry Communications","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1388248124001255","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ELECTROCHEMISTRY","Score":null,"Total":0}
引用次数: 0
摘要
本研究探讨了高熵合金 (HEA) 作为催化剂降低质子交换膜燃料电池 (PEMFC) 中氧还原反应 (ORR) 能量障碍的有效性。对四种高熵合金--铱钯铂铬、钴铬铁镍、铌钼钽钨和钛锌锆铌钽--作为潜在催化剂进行了分析。这种优越性源于 HEA 中整个 d 波段中心位置向负能量的转移。研究表明,HEAs 中原子价标准偏差的增加与 ORR 效率的提高呈正相关,这表明它是具有成本效益的催化剂的潜在设计指标。此外,还提出了基于单个元素之间电负性差异的化合价变化预测。此外,研究还强调,在 HEA 上增加铂的表面吸附将进一步提高 ORR 活性。
Mitigating oxygen reduction reaction barriers: An in-depth first-principles exploration of high-entropy alloy as catalysts
This study investigates the effectiveness of high-entropy alloys (HEAs) as catalysts for reducing the energy barrier of the oxygen reduction reaction (ORR) in proton exchange membrane fuel cells (PEMFCs). Four HEAs—IrPdPtRh, CoCrFeNi, NbMoTaW, and TiZrNbTa—are analyzed as potential catalysts. This superiority arises from the shift in the overall d-band center position towards negative energy in HEAs. The study suggests that an increased standard deviation of atomic valences within HEAs correlates positively with improved ORR efficiency, indicating it as a potential design indicator for cost-effective catalysts. Moreover, predictions of valence variations based on differences in electronegativity between individual elements are proposed. Additionally, the research highlights that additional surface adsorption of Pt on HEAs would further enhance ORR activity.
期刊介绍:
Electrochemistry Communications is an open access journal providing fast dissemination of short communications, full communications and mini reviews covering the whole field of electrochemistry which merit urgent publication. Short communications are limited to a maximum of 20,000 characters (including spaces) while full communications and mini reviews are limited to 25,000 characters (including spaces). Supplementary information is permitted for full communications and mini reviews but not for short communications. We aim to be the fastest journal in electrochemistry for these types of papers.