{"title":"全球海洋环境中丙烯酸树脂涂料老化严重程度的预测绘图和分析","authors":"Haodi Ji, Xiaobing Ma, Yikun Cai, Shuo Jiao","doi":"10.1007/s10853-024-09999-2","DOIUrl":null,"url":null,"abstract":"<div><p>The aging failure process of acrylic resin (AR) coatings widely used in ship anti-corrosion systems is highly complex. Currently, there are no established models or methods for predicting the aging of AR coatings in different marine environments. Therefore, this study proposes a framework for predicting the aging of AR coatings in marine environment based on short-term indoor accelerated tests. Initially, a comprehensive aging evaluation method for AR coatings is developed by integrating three commonly used coating performance evaluation indicators (gloss, color difference, and electrochemical impedance) based on the Technique for Order Preference by Similarity to Ideal Solution. Subsequently, an aging severity index is defined to quantify the impact of different environments on the coating aging process. Following this, 14 sets of indoor accelerated aging tests for AR coatings under various environmental conditions are conducted. Based on the test results, a comparative analysis of the predictive performance of three environmental effect models, namely multiple linear regression model, generalized Eyring model, and genetic algorithm-back-propagation model, is performed. Finally, utilizing the environmental effect models and global marine environmental data, the aging severity index of AR coatings in global marine environments is predicted and extrapolated.</p></div>","PeriodicalId":645,"journal":{"name":"Journal of Materials Science","volume":"59 31","pages":"14790 - 14806"},"PeriodicalIF":3.9000,"publicationDate":"2024-07-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Predictive mapping and analysis of aging severity for acrylic resin coatings in global marine environments\",\"authors\":\"Haodi Ji, Xiaobing Ma, Yikun Cai, Shuo Jiao\",\"doi\":\"10.1007/s10853-024-09999-2\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The aging failure process of acrylic resin (AR) coatings widely used in ship anti-corrosion systems is highly complex. Currently, there are no established models or methods for predicting the aging of AR coatings in different marine environments. Therefore, this study proposes a framework for predicting the aging of AR coatings in marine environment based on short-term indoor accelerated tests. Initially, a comprehensive aging evaluation method for AR coatings is developed by integrating three commonly used coating performance evaluation indicators (gloss, color difference, and electrochemical impedance) based on the Technique for Order Preference by Similarity to Ideal Solution. Subsequently, an aging severity index is defined to quantify the impact of different environments on the coating aging process. Following this, 14 sets of indoor accelerated aging tests for AR coatings under various environmental conditions are conducted. Based on the test results, a comparative analysis of the predictive performance of three environmental effect models, namely multiple linear regression model, generalized Eyring model, and genetic algorithm-back-propagation model, is performed. Finally, utilizing the environmental effect models and global marine environmental data, the aging severity index of AR coatings in global marine environments is predicted and extrapolated.</p></div>\",\"PeriodicalId\":645,\"journal\":{\"name\":\"Journal of Materials Science\",\"volume\":\"59 31\",\"pages\":\"14790 - 14806\"},\"PeriodicalIF\":3.9000,\"publicationDate\":\"2024-07-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Materials Science\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10853-024-09999-2\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Materials Science","FirstCategoryId":"88","ListUrlMain":"https://link.springer.com/article/10.1007/s10853-024-09999-2","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
广泛用于船舶防腐系统的丙烯酸树脂(AR)涂料的老化失效过程非常复杂。目前,还没有成熟的模型或方法来预测 AR 涂料在不同海洋环境中的老化。因此,本研究提出了一个基于短期室内加速试验的海洋环境 AR 涂层老化预测框架。首先,基于与理想解相似性排序优先技术,通过整合三个常用的涂层性能评价指标(光泽度、色差和电化学阻抗),建立了 AR 涂层的综合老化评价方法。随后,定义了老化严重程度指数,以量化不同环境对涂层老化过程的影响。随后,对 AR 涂层在不同环境条件下进行了 14 组室内加速老化试验。根据试验结果,对三种环境效应模型(即多元线性回归模型、广义艾林模型和遗传算法-反向传播模型)的预测性能进行了比较分析。最后,利用环境效应模型和全球海洋环境数据,预测和推断了 AR 涂层在全球海洋环境中的老化严重指数。
Predictive mapping and analysis of aging severity for acrylic resin coatings in global marine environments
The aging failure process of acrylic resin (AR) coatings widely used in ship anti-corrosion systems is highly complex. Currently, there are no established models or methods for predicting the aging of AR coatings in different marine environments. Therefore, this study proposes a framework for predicting the aging of AR coatings in marine environment based on short-term indoor accelerated tests. Initially, a comprehensive aging evaluation method for AR coatings is developed by integrating three commonly used coating performance evaluation indicators (gloss, color difference, and electrochemical impedance) based on the Technique for Order Preference by Similarity to Ideal Solution. Subsequently, an aging severity index is defined to quantify the impact of different environments on the coating aging process. Following this, 14 sets of indoor accelerated aging tests for AR coatings under various environmental conditions are conducted. Based on the test results, a comparative analysis of the predictive performance of three environmental effect models, namely multiple linear regression model, generalized Eyring model, and genetic algorithm-back-propagation model, is performed. Finally, utilizing the environmental effect models and global marine environmental data, the aging severity index of AR coatings in global marine environments is predicted and extrapolated.
期刊介绍:
The Journal of Materials Science publishes reviews, full-length papers, and short Communications recording original research results on, or techniques for studying the relationship between structure, properties, and uses of materials. The subjects are seen from international and interdisciplinary perspectives covering areas including metals, ceramics, glasses, polymers, electrical materials, composite materials, fibers, nanostructured materials, nanocomposites, and biological and biomedical materials. The Journal of Materials Science is now firmly established as the leading source of primary communication for scientists investigating the structure and properties of all engineering materials.