反应相分离系统中的复杂动力学

Dino Osmanovic, Elisa Franco
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引用次数: 0

摘要

我们研究了反应相分离系统中出现的持续时空行为。我们将重点放在二元系统上,其中一个或两个物种可以相分离,我们讨论了决定霍普夫型分叉出现条件的均相状态的稳定性。然后,我们研究了特定自催化化学反应的影响,并通过计算确定了偏微分方程的全解。我们发现,当两个物种相分离时,在一维中会出现持续的脉冲动力学。当在二维中考虑时,系统会产生持续、复杂的动态液滴,而如果只有一个物种可以相分离,则一般不会出现这种情况。最后,我们讨论了具有复杂特征的动力学的出现,这可以用细胞自动机的框架来理解。
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Complex Dynamics in Reaction-Phase Separation Systems
We investigate the emergence of sustained spatio-temporal behaviors in reaction-phase separation systems. We focus on binary systems, in which either one or both species can phase separate, and we discuss the stability of the homogeneous state determining the conditions for the emergence of a Hopf-type bifurcation. We then examine the effects of a specific autocatalytic chemical reaction, and computationally determine the full solutions to the partial differential equations. We find that when both species phase separate, sustained pulsed dynamics arise in one dimension. When considered in two dimensions, the system generates persistent, complex dynamic droplets, which do not generally appear if only one of the species can phase separate. We finally discuss the emergence of dynamics with complex features, which can be understood using the framework of a cellular automata.
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