消除氮氧化物(NOx)和挥发性有机化合物(VOC)的沸石基材料:进展与未来展望

IF 5.4 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2024-08-27 DOI:10.1039/d4cy00841c
Xiaoli Zhu , Ying Xin , Long Yu , Shuai Liu , Dongxu Han , Junxiu Jia , Jin Wang , Zhaoliang Zhang
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引用次数: 0

摘要

随着环保意识的增强,人们最为关注的一个密不可分的问题就是大气污染。其中,氮氧化物(NOx)和挥发性有机化合物(VOCs)等主要气态污染物是形成细颗粒物和臭氧的前体物质,已引起人们的极大关注。为了消除这些污染物,沸石基材料因其显著的形状选择性、吸附和离子交换能力、高水热耐久性、可调的酸度和极性以及低廉的生产成本,已成为不可或缺的吸附剂和/或催化剂。此外,改变它们的多孔结构和组成,并加入外来物种,可在各种具有挑战性的环境治理过程中实现前所未有的高性能。在这一视角中,我们将重点关注利用沸石材料消除氮氧化物和挥发性有机化合物的最新进展。特别是阐明了多孔结构和成分对吸附和催化转化性能的影响。最后,确定并概述了利用沸石基材料的潜在挑战和未来机遇,以满足未来对改善大气环境日益增长的要求。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Zeolite-based materials eliminating nitrogen oxides (NOx) and volatile organic compounds (VOCs): advances and future perspectives

As awareness of environmental protection increases, the most inextricably linked issue of greatest concern is atmospheric pollution. In particular, the major gaseous pollutants, such as nitrogen oxides (NOx) and volatile organic compounds (VOCs), which are the precursors for the formation of fine particulate matter and ozone, have attracted significant attention. To eliminate these pollutants, zeolite-based materials have become the indispensable adsorbents and/or catalysts due to their remarkable shape selectivity, adsorption and ion exchange capability, high hydrothermal durability, tunable acidity and polarity, and affordable production expenses. Furthermore, modifying their porous architectures and compositions, and the incorporation of exotic species could lead to an unprecedented high performance in a wide range of challenging environmental governance processes. In this perspective, we focus on the latest advancements in employing zeolite-based materials to eliminate NOx and VOCs. Especially, the impacts of porous structures and components on the performance of adsorption and catalytic conversion were elucidated. Finally, the potential challenges and future opportunities for the utilization of zeolite-based materials are identified and outlined to meet the ever-increasing requirements for the improved atmospheric environment in the future.

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来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
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