Soyeun Kim, Gal Orenstein, Anisha G Singh, Ian R Fisher, David A Reis, Mariano Trigo
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引用次数: 0
摘要
我们报告了对各向异性应变下碲化镉(TbTe3)中电荷密度波(CDW)阶次参数动态的超快反射率测量结果。我们观察到振幅模式的频率随着沿 a 轴的拉伸应变的增加而增加(拉伸应变使晶格的 a>c,a 和 c 为晶格常数),沿 c 轴的拉伸应变也有类似的表现(c>a)。这表明,尽管存在正交空间群,但这两种应变都能稳定相应的 CDW 阶次,并进一步证明了在 a 轴和 c 轴方向上的 CDW 相几乎等同。应变依赖性表明,正交 a 和 c CDW 分别在相应的 a > c 和 c > a 应变下稳定。我们的研究提出了一种超快方法来评估应变系统中相的稳定性和有序参数动态。
Emergent symmetry in TbTe3revealed by ultrafast reflectivity under anisotropic strain.
We report ultrafast reflectivity measurements of the dynamics of the order parameter of the charge density wave (CDW) in TbTe3under anisotropic strain. We observe an increase in the frequency of the amplitude mode with increasing tensile strain along thea-axis (which drives the lattice intoa > c, withaandcthe lattice constants), and similar behavior for tensile strain alongc(c > a). This suggests that both strains stabilize the corresponding CDW order and further support the near equivalence of the CDW phases oriented ina- andc-axis, in spite of the orthorhombic space group. The results were analyzed within the time-dependent Ginzburg-Landau framework, which agrees well with the reflectivity dynamics. Our study presents an ultrafast approach to assess the stability of phases and order parameter dynamics in strained systems.