沿中子数 N = 50 从 78Ni 到 70Ca 的 Ab initio 计算

IF 5.4 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2024-09-11 DOI:10.1016/j.physletb.2024.139010
B.S. Hu , Z.H. Sun , G. Hagen , G.R. Jansen , T. Papenbrock
{"title":"沿中子数 N = 50 从 78Ni 到 70Ca 的 Ab initio 计算","authors":"B.S. Hu ,&nbsp;Z.H. Sun ,&nbsp;G. Hagen ,&nbsp;G.R. Jansen ,&nbsp;T. Papenbrock","doi":"10.1016/j.physletb.2024.139010","DOIUrl":null,"url":null,"abstract":"<div><p>We present coupled-cluster computations of nuclei with neutron number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> “south” of <sup>78</sup>Ni using nucleon-nucleon and three-nucleon forces from chiral effective field theory. We find an erosion of the magic number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> toward <sup>70</sup>Ca manifesting itself by an onset of deformation and increased complexity in the ground states. For <sup>78</sup>Ni, we predict a low-lying rotational band consistent with recent data, which up until now has been a challenge for ab initio nuclear models. Ground states are deformed in <sup>76</sup>Fe, <sup>74</sup>Cr, and <sup>72</sup>Ti, although the spherical states are too close in energy to unambiguously identify the shape of the ground state within the uncertainty estimates. In <sup>70</sup>Ca, the potential energy landscape from quadrupole-constrained Hartree-Fock computations flattens, and the deformation becomes less rigid. We also compute the low-lying spectra and <span><math><mi>B</mi><mo>(</mo><mi>E</mi><mn>2</mn><mo>)</mo></math></span> values for these neutron-rich <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> nuclei.</p></div>","PeriodicalId":4,"journal":{"name":"ACS Applied Energy Materials","volume":null,"pages":null},"PeriodicalIF":5.4000,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0370269324005689/pdfft?md5=1fd0998cb302fbbe296f8a5b4c580252&pid=1-s2.0-S0370269324005689-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Ab initio computations from 78Ni towards 70Ca along neutron number N = 50\",\"authors\":\"B.S. Hu ,&nbsp;Z.H. Sun ,&nbsp;G. Hagen ,&nbsp;G.R. Jansen ,&nbsp;T. Papenbrock\",\"doi\":\"10.1016/j.physletb.2024.139010\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>We present coupled-cluster computations of nuclei with neutron number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> “south” of <sup>78</sup>Ni using nucleon-nucleon and three-nucleon forces from chiral effective field theory. We find an erosion of the magic number <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> toward <sup>70</sup>Ca manifesting itself by an onset of deformation and increased complexity in the ground states. For <sup>78</sup>Ni, we predict a low-lying rotational band consistent with recent data, which up until now has been a challenge for ab initio nuclear models. Ground states are deformed in <sup>76</sup>Fe, <sup>74</sup>Cr, and <sup>72</sup>Ti, although the spherical states are too close in energy to unambiguously identify the shape of the ground state within the uncertainty estimates. In <sup>70</sup>Ca, the potential energy landscape from quadrupole-constrained Hartree-Fock computations flattens, and the deformation becomes less rigid. We also compute the low-lying spectra and <span><math><mi>B</mi><mo>(</mo><mi>E</mi><mn>2</mn><mo>)</mo></math></span> values for these neutron-rich <span><math><mi>N</mi><mo>=</mo><mn>50</mn></math></span> nuclei.</p></div>\",\"PeriodicalId\":4,\"journal\":{\"name\":\"ACS Applied Energy Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2024-09-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S0370269324005689/pdfft?md5=1fd0998cb302fbbe296f8a5b4c580252&pid=1-s2.0-S0370269324005689-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Energy Materials\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0370269324005689\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Energy Materials","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0370269324005689","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0

摘要

我们利用手性有效场理论中的核子-核子力和三核子力,对 78Ni "以南 "中子数 N=50 的原子核进行了耦合-簇计算。我们发现神奇数字 N=50 在向 70Ca 移动的过程中会受到侵蚀,表现为基态开始变形,复杂性增加。对于 78Ni,我们预测出了一个与最新数据相一致的低洼旋转带,到目前为止,这一直是原子核模型所面临的挑战。在 76Fe、74Cr 和 72Ti 中,基态发生了变形,尽管球形态的能量过于接近,无法在不确定性估计范围内明确确定基态的形状。在 70Ca 中,四极约束哈特里-福克(Hartree-Fock)计算得出的势能图变得平缓,变形也变得不那么刚硬。我们还计算了这些富中子 N=50 核的低洼谱和 B(E2) 值。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Ab initio computations from 78Ni towards 70Ca along neutron number N = 50

We present coupled-cluster computations of nuclei with neutron number N=50 “south” of 78Ni using nucleon-nucleon and three-nucleon forces from chiral effective field theory. We find an erosion of the magic number N=50 toward 70Ca manifesting itself by an onset of deformation and increased complexity in the ground states. For 78Ni, we predict a low-lying rotational band consistent with recent data, which up until now has been a challenge for ab initio nuclear models. Ground states are deformed in 76Fe, 74Cr, and 72Ti, although the spherical states are too close in energy to unambiguously identify the shape of the ground state within the uncertainty estimates. In 70Ca, the potential energy landscape from quadrupole-constrained Hartree-Fock computations flattens, and the deformation becomes less rigid. We also compute the low-lying spectra and B(E2) values for these neutron-rich N=50 nuclei.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
期刊最新文献
Red ginseng polysaccharide promotes ferroptosis in gastric cancer cells by inhibiting PI3K/Akt pathway through down-regulation of AQP3. Diagnostic value of 18F-PSMA-1007 PET/CT for predicting the pathological grade of prostate cancer. Correction. Wilms' tumor 1 -targeting cancer vaccine: Recent advancements and future perspectives. Toll-like receptor agonists as cancer vaccine adjuvants.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1