{"title":"在绿色溶剂水/乙醇混合物液滴上进行双染双色激光诱导荧光光谱分析,以测定温度和混合物成分","authors":"Hannah Ulrich, Richard Weiß, Lars Zigan","doi":"10.1007/s00348-024-03868-z","DOIUrl":null,"url":null,"abstract":"<div><p>This work shows new insights on the application of two-color laser-induced-fluorescence (2c-LIF) thermometry in a droplet chain. A two-dye mixture is used in ethanol, water and ethanol/water mixtures in order to reach a high-temperature sensitivity and avoid the detection of lasing effects in the droplets. Various droplet sizes are recorded in regard to the limitation of the detection system for very small micrometric droplets. The breakup of a droplet chain is measured to assess the spectral detection system in applications with liquid structures of different sizes. Additionally, a proposal to expand the 2c-LIF application for studying ethanol/water droplets regarding mixture composition with a third color channel is presented. Forming two intensity ratios, the spectra can be used to obtain information on the mixture composition of the solvent. Measurements in different ethanol/water mixtures containing 0–100 vol% water are evaluated to show this possibility.</p></div>","PeriodicalId":554,"journal":{"name":"Experiments in Fluids","volume":"65 9","pages":""},"PeriodicalIF":2.3000,"publicationDate":"2024-08-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s00348-024-03868-z.pdf","citationCount":"0","resultStr":"{\"title\":\"Two-dye two-color laser-induced fluorescence spectroscopy on droplets of green solvent water/ethanol mixtures for thermometry and mixture composition\",\"authors\":\"Hannah Ulrich, Richard Weiß, Lars Zigan\",\"doi\":\"10.1007/s00348-024-03868-z\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>This work shows new insights on the application of two-color laser-induced-fluorescence (2c-LIF) thermometry in a droplet chain. A two-dye mixture is used in ethanol, water and ethanol/water mixtures in order to reach a high-temperature sensitivity and avoid the detection of lasing effects in the droplets. Various droplet sizes are recorded in regard to the limitation of the detection system for very small micrometric droplets. The breakup of a droplet chain is measured to assess the spectral detection system in applications with liquid structures of different sizes. Additionally, a proposal to expand the 2c-LIF application for studying ethanol/water droplets regarding mixture composition with a third color channel is presented. Forming two intensity ratios, the spectra can be used to obtain information on the mixture composition of the solvent. Measurements in different ethanol/water mixtures containing 0–100 vol% water are evaluated to show this possibility.</p></div>\",\"PeriodicalId\":554,\"journal\":{\"name\":\"Experiments in Fluids\",\"volume\":\"65 9\",\"pages\":\"\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2024-08-20\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://link.springer.com/content/pdf/10.1007/s00348-024-03868-z.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Experiments in Fluids\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s00348-024-03868-z\",\"RegionNum\":3,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENGINEERING, MECHANICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Experiments in Fluids","FirstCategoryId":"5","ListUrlMain":"https://link.springer.com/article/10.1007/s00348-024-03868-z","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, MECHANICAL","Score":null,"Total":0}
Two-dye two-color laser-induced fluorescence spectroscopy on droplets of green solvent water/ethanol mixtures for thermometry and mixture composition
This work shows new insights on the application of two-color laser-induced-fluorescence (2c-LIF) thermometry in a droplet chain. A two-dye mixture is used in ethanol, water and ethanol/water mixtures in order to reach a high-temperature sensitivity and avoid the detection of lasing effects in the droplets. Various droplet sizes are recorded in regard to the limitation of the detection system for very small micrometric droplets. The breakup of a droplet chain is measured to assess the spectral detection system in applications with liquid structures of different sizes. Additionally, a proposal to expand the 2c-LIF application for studying ethanol/water droplets regarding mixture composition with a third color channel is presented. Forming two intensity ratios, the spectra can be used to obtain information on the mixture composition of the solvent. Measurements in different ethanol/water mixtures containing 0–100 vol% water are evaluated to show this possibility.
期刊介绍:
Experiments in Fluids examines the advancement, extension, and improvement of new techniques of flow measurement. The journal also publishes contributions that employ existing experimental techniques to gain an understanding of the underlying flow physics in the areas of turbulence, aerodynamics, hydrodynamics, convective heat transfer, combustion, turbomachinery, multi-phase flows, and chemical, biological and geological flows. In addition, readers will find papers that report on investigations combining experimental and analytical/numerical approaches.