在聚吡咯@单面绒布上实现高效太阳能驱动的界面水蒸发

IF 4.8 Q1 ENVIRONMENTAL SCIENCES ACS ES&T water Pub Date : 2024-08-29 DOI:10.1021/acsestwater.4c0070810.1021/acsestwater.4c00708
Tian Wu, Wanhui Shi, Yunzhen Chang, Ying Zhang, Yue Zhang, Yanping Li, Sheng Zhu*, Fengzhen Yuan and Gaoyi Han*, 
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引用次数: 0

摘要

太阳能界面蒸发被认为是解决全球淡水短缺问题的一项创新而有效的技术,其有效性主要取决于光热材料的效率。在此,我们设计了一种太阳能蒸发装置,由用于收集水的海绵层和化学沉积在单面绒布上用于吸收阳光的聚吡咯(PPy)层(PPy@SSF)组成。PPy@SSF 中的纤维阵列有助于吸收光能,在光吸收层和水之间建立一个加热界面。海绵层不仅有助于集水,还可作为隔热层,防止热量散失。由此产生的装置具有水蒸发量大、稳定性强、耐盐碱等特点。在阳光直射下,日出水量达到 8.12 kg m-2。在对模拟海水进行脱盐处理时,冷凝水中的离子浓度降低了 4 个数量级。此外,污水净化水中的重金属离子也减少了至少 3 个数量级。此外,在 1 个太阳下反复使用 10 次后,该装置的性能也没有衰减。我们的研究为海水和污水净化提供了一个具有高光热转换效率的平台。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Highly Efficient Solar-Driven Interface Water Evaporation Achieved on Polypyrrole@Single-Sided Flannel

Solar interface evaporation is considered an innovative and effective technology for combating global freshwater scarcity, with its effectiveness primarily hinging on the efficiency of photothermal materials. Here, we designed a solar evaporation device comprising a sponge layer for water collection and a polypyrrole (PPy) layer chemically deposited on a single-sided flannel (PPy@SSF) for sunlight absorption. The fiber array within PPy@SSF facilitates to absorb light energy, establishing a heating interface between the light absorption layer and the water. The sponge layer not only aids in water collection but also serves as a thermal insulation layer, preventing heat dispersion. The resulting device exhibits characteristics such as high water evaporation, robust stability, and resistance to salt. The daily water output reaches 8.12 kg m–2 under direct sunlight. In desalinating simulated seawater, the ion concentrations in the condensed water were reduced by 4 orders. Furthermore, heavy metal ions in purified water from sewage were reduced by at least 3 orders of magnitude. Additionally, the properties of the device showed no attenuation after being used repeatedly 10 times under 1 sun. Our research provides a platform with high photothermal conversion efficiency for seawater and sewage purification.

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