以煤为原料的气化 SNG 热电联产与钙循环相结合,提高二氧化碳吸收率

Yuan, Chen, Can, Deng, Jingyuan, Zhu, Bingyang, Du, Rui, Zhang, Ziyu, Li, Huimin, Liu
{"title":"以煤为原料的气化 SNG 热电联产与钙循环相结合,提高二氧化碳吸收率","authors":"Yuan, Chen, Can, Deng, Jingyuan, Zhu, Bingyang, Du, Rui, Zhang, Ziyu, Li, Huimin, Liu","doi":"10.26434/chemrxiv-2024-grhpq","DOIUrl":null,"url":null,"abstract":"This paper studies the conversion of coal to energy vectors (power and SNG) through gasification simultaneously with a chemical looping process from a thermodynamic perspective. Water-gas shift with calcium looping CO2 absorption process is conducted as the substitute of traditional water-gas shift reaction (WGS) with amine sorbents. This novel technology includes six main parts: cryogenic air separation unit (CASU), coal gasification, the water-gas shift process with calcium looping for enhancement of CO2 absorption (WGS-CaL), methanation and heat recovery steam generation (HRSG). WGS-CaL is an efficient method for adjusting the ratio of CO and H2 as well as CO2 capturing. The simulation results are consistent with the industrial data. Moreover, the overall plant energy and economic performance are compared with traditional carbon capture technologies.","PeriodicalId":9813,"journal":{"name":"ChemRxiv","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Gasification for SNG-power cogeneration using coal as material integrated with calcium looping for enhancing CO2 absorption\",\"authors\":\"Yuan, Chen, Can, Deng, Jingyuan, Zhu, Bingyang, Du, Rui, Zhang, Ziyu, Li, Huimin, Liu\",\"doi\":\"10.26434/chemrxiv-2024-grhpq\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"This paper studies the conversion of coal to energy vectors (power and SNG) through gasification simultaneously with a chemical looping process from a thermodynamic perspective. Water-gas shift with calcium looping CO2 absorption process is conducted as the substitute of traditional water-gas shift reaction (WGS) with amine sorbents. This novel technology includes six main parts: cryogenic air separation unit (CASU), coal gasification, the water-gas shift process with calcium looping for enhancement of CO2 absorption (WGS-CaL), methanation and heat recovery steam generation (HRSG). WGS-CaL is an efficient method for adjusting the ratio of CO and H2 as well as CO2 capturing. The simulation results are consistent with the industrial data. Moreover, the overall plant energy and economic performance are compared with traditional carbon capture technologies.\",\"PeriodicalId\":9813,\"journal\":{\"name\":\"ChemRxiv\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-09-18\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ChemRxiv\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.26434/chemrxiv-2024-grhpq\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ChemRxiv","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.26434/chemrxiv-2024-grhpq","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

摘要

本文从热力学角度研究了煤炭通过气化与化学循环过程同时转化为能源载体(电力和合成天然气)的过程。水煤气变换与钙循环二氧化碳吸收工艺是以胺吸附剂替代传统的水煤气变换反应(WGS)。这项新技术包括六个主要部分:低温空分装置(CASU)、煤气化、水煤气变换工艺与钙循环以提高二氧化碳吸收率(WGS-CaL)、甲烷化和热回收蒸汽发生器(HRSG)。WGS-CaL 是调整 CO 和 H2 比例以及捕获 CO2 的有效方法。模拟结果与工业数据一致。此外,还将整个工厂的能源和经济效益与传统的碳捕集技术进行了比较。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Gasification for SNG-power cogeneration using coal as material integrated with calcium looping for enhancing CO2 absorption
This paper studies the conversion of coal to energy vectors (power and SNG) through gasification simultaneously with a chemical looping process from a thermodynamic perspective. Water-gas shift with calcium looping CO2 absorption process is conducted as the substitute of traditional water-gas shift reaction (WGS) with amine sorbents. This novel technology includes six main parts: cryogenic air separation unit (CASU), coal gasification, the water-gas shift process with calcium looping for enhancement of CO2 absorption (WGS-CaL), methanation and heat recovery steam generation (HRSG). WGS-CaL is an efficient method for adjusting the ratio of CO and H2 as well as CO2 capturing. The simulation results are consistent with the industrial data. Moreover, the overall plant energy and economic performance are compared with traditional carbon capture technologies.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
0
期刊最新文献
Exascale Quantum Mechanical Simulations: Navigating the Shifting Sands of Hardware and Software Hybrid synthesis of AMFC-derived amides using supported gold nanoparticles and acyl-coenzyme A ligases Non-covalent spin labelling of TRPC5 ion channels enables EPR studies of protein-ligand interactions An Efficient RI-MP2 Algorithm for Distributed Many-GPU Architectures Unusual Confinement-Induced Basicity and Proton-Mediated CH Activity of an Adipic Acid-Ammonium Cluster
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1