高压下氨/氢/空气湍流预混合火焰燃烧速度的实验研究

IF 5.2 3区 工程技术 Q2 ENERGY & FUELS Energy & Fuels Pub Date : 2024-09-11 DOI:10.1021/acs.energyfuels.4c0294210.1021/acs.energyfuels.4c02942
Jian-Bin Cao, Jun-Qiang Ma, Guo-Xiu Li*, Hong-Meng Li* and Rong-Pei Jiang*, 
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引用次数: 0

摘要

在一个能够产生各向同性均匀湍流场的燃烧器中研究了氨/氢/空气混合物的预混合火焰。根据不同氢比、湍流强度和路易斯数约为 1 的压力下的传播特性,分析了火焰化学性质、湍流伸展和压力对湍流燃烧速度的影响。结果表明,湍流强度能显著增强火焰的传播,而压力的影响在不同湍流条件下各不相同,氢比对应于火焰化学性质的增强,对火焰传播有很大影响。压力和湍流强度的增加使火焰的卡洛维兹数增大,从而容易受到湍流拉伸的影响。此外,湍流火焰表现出明显的自相似加速传播,但当氢比较大时,拟合指数存在偏差。此外,考虑到压力对燃烧过程的影响,本文研究了高压下湍流燃烧速度的几种相关性,并在这些相关性中引入归一化压力和湍流积分长度尺度进行深入分析,然后进一步讨论了现有相关性的局限性。
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Experimental Investigation on Burning Velocity of Ammonia/Hydrogen/Air Turbulent Premixed Flames under Elevated Pressure

Premixed flames of ammonia/hydrogen/air mixtures were investigated in a combustor capable of creating an isotropic and homogeneous turbulent field. Based on the propagation characteristics under different hydrogen ratios, turbulence intensities, and pressures with Lewis numbers of about 1, the effects of flame chemistry, turbulent stretch, and pressure on the turbulent burning velocity were analyzed. The results show that turbulence intensity can significantly enhance the flame propagation, while the effect of pressure varies under different turbulence conditions and the hydrogen ratio corresponds to the enhancement of the flame chemistry, which has a great influence on the flame propagation. The increase of pressure and turbulence intensity makes the flame have a larger Karlovitz number and thus susceptible to turbulent stretching. In addition, the turbulent flame shows obvious self-similar accelerated propagation, but there is a deviation in the fitting index when the hydrogen ratio is larger. In addition, considering the effect of pressure on the combustion process, this paper studies the applicability of several correlations for turbulent burning velocity under high pressure and introduces the normalized pressure and turbulence integral length scales into these correlations for in-depth analysis and then further discusses the limitations of the existing correlations.

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来源期刊
Energy & Fuels
Energy & Fuels 工程技术-工程:化工
CiteScore
9.20
自引率
13.20%
发文量
1101
审稿时长
2.1 months
期刊介绍: Energy & Fuels publishes reports of research in the technical area defined by the intersection of the disciplines of chemistry and chemical engineering and the application domain of non-nuclear energy and fuels. This includes research directed at the formation of, exploration for, and production of fossil fuels and biomass; the properties and structure or molecular composition of both raw fuels and refined products; the chemistry involved in the processing and utilization of fuels; fuel cells and their applications; and the analytical and instrumental techniques used in investigations of the foregoing areas.
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