{"title":"在钚生产的辅助下,利用 COMPRE 方法评估 SMR 的抗增殖能力","authors":"Kwangho Ju , SeoungHo Jeong , Hosik Yoo","doi":"10.1016/j.nucengdes.2024.113615","DOIUrl":null,"url":null,"abstract":"<div><div>The proliferation resistance (PR) of several small modular reactors (SMR) is investigated in terms of material characteristic and other extrinsic parameters with COMPRE methodology developed by KINAC. In this work, plutonium (Pu) production amount and isotopic yield are newly introduced as key metrics in material characteristic. Their functionalization is performed with a linear regression method based on sparse core depletion data. Nevertheless, a clear discrepancy is observed in Pu buildup and its quality depending on SMR type and core burnup status. Some of the non-light water SMRs exhibit a higher proliferation concern and their PR score trends are clearly different compared to conventional pressurized water reactors (PWR). Other extrinsic parameters are evaluated based on development status of representative SMRs. At present, liquid metal cooled-fast reactor (LMFR) and molten salt reactor (MSR) receive low scores due to their limited technical maturity in reactor design and related I&C equipment. We conclude that distinct safeguards approaches, suitable for a wide range of SMR designs should be developed for commercial use in the near future.</div></div>","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Evaluation of proliferation resistance of SMRs with COMPRE methodology assisted by Pu production\",\"authors\":\"Kwangho Ju , SeoungHo Jeong , Hosik Yoo\",\"doi\":\"10.1016/j.nucengdes.2024.113615\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The proliferation resistance (PR) of several small modular reactors (SMR) is investigated in terms of material characteristic and other extrinsic parameters with COMPRE methodology developed by KINAC. In this work, plutonium (Pu) production amount and isotopic yield are newly introduced as key metrics in material characteristic. Their functionalization is performed with a linear regression method based on sparse core depletion data. Nevertheless, a clear discrepancy is observed in Pu buildup and its quality depending on SMR type and core burnup status. Some of the non-light water SMRs exhibit a higher proliferation concern and their PR score trends are clearly different compared to conventional pressurized water reactors (PWR). Other extrinsic parameters are evaluated based on development status of representative SMRs. At present, liquid metal cooled-fast reactor (LMFR) and molten salt reactor (MSR) receive low scores due to their limited technical maturity in reactor design and related I&C equipment. We conclude that distinct safeguards approaches, suitable for a wide range of SMR designs should be developed for commercial use in the near future.</div></div>\",\"PeriodicalId\":1,\"journal\":{\"name\":\"Accounts of Chemical Research\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":16.4000,\"publicationDate\":\"2024-10-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Accounts of Chemical Research\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0029549324007155\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0029549324007155","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
Evaluation of proliferation resistance of SMRs with COMPRE methodology assisted by Pu production
The proliferation resistance (PR) of several small modular reactors (SMR) is investigated in terms of material characteristic and other extrinsic parameters with COMPRE methodology developed by KINAC. In this work, plutonium (Pu) production amount and isotopic yield are newly introduced as key metrics in material characteristic. Their functionalization is performed with a linear regression method based on sparse core depletion data. Nevertheless, a clear discrepancy is observed in Pu buildup and its quality depending on SMR type and core burnup status. Some of the non-light water SMRs exhibit a higher proliferation concern and their PR score trends are clearly different compared to conventional pressurized water reactors (PWR). Other extrinsic parameters are evaluated based on development status of representative SMRs. At present, liquid metal cooled-fast reactor (LMFR) and molten salt reactor (MSR) receive low scores due to their limited technical maturity in reactor design and related I&C equipment. We conclude that distinct safeguards approaches, suitable for a wide range of SMR designs should be developed for commercial use in the near future.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.