光悬浮液滴团数量依赖性自组装模式的新见解。

IF 2.7 2区 化学 Q3 CHEMISTRY, PHYSICAL The Journal of Physical Chemistry A Pub Date : 2024-10-31 Epub Date: 2024-10-16 DOI:10.1021/acs.jpca.4c06443
Pengcheng Jiang, Yijing Yang, Xun Zhu, Dingding Ye, Yang Yang, Hong Wang, Liang An, Alexander A Fedorets, Qiang Liao, Rong Chen, Michael Nosonovsky
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引用次数: 0

摘要

据报道,热气-液界面上方的轻悬浮液滴团的自组装模式取决于液滴的数量。然而,当光悬浮液滴的数量超过 15 个时,已报道的关于数量依赖性自组装模式的理论解释就不能很好地发挥作用。在此,我们提出了一个新的理论视角,即通过引入最小总势能原理,参照经典的大圆中相同刚性圆的最密堆积问题,来理解轻悬液滴团的自组装。令人惊奇的是,尽管轻悬液滴的数量多达 142 个,但这种新方法得到的理论结果与实验结果非常吻合。这项研究加深了我们对光悬浮液滴团数量依赖性自组装模式的理解,并为其他类似的自组装现象提供了重要启示。
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New Insight into Quantity-Dependent Self-Assembly Pattern of Light Levitating Droplet Clusters.

It has been reported that the self-assembly pattern of light levitating droplet clusters above the hot gas-liquid interface is dependent on the quantity of droplets. However, the already-reported theoretical explanation of the quantity-dependent self-assembly pattern cannot work well when the quantity of the light levitating droplet exceeds 15. Herein, we propose a new theoretical perspective to understand the self-assembly of a light levitating droplet cluster by referring to the classical densest packing problem of identical rigid circles in a larger circle with the introduction of the minimum total potential energy principle. Amazingly, the theoretical results obtained by this new approach agree well with experimental results, even though the quantity of the light levitating droplet is up to 142. This study deepens our understanding of the quantity-dependent self-assembly pattern of the light levitating droplet clusters and provides significant inspiration for other analogous self-assembly phenomena.

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来源期刊
The Journal of Physical Chemistry A
The Journal of Physical Chemistry A 化学-物理:原子、分子和化学物理
CiteScore
5.20
自引率
10.30%
发文量
922
审稿时长
1.3 months
期刊介绍: The Journal of Physical Chemistry A is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, and chemical physicists.
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