Hyunmin Hong, Min Jung Kim, Dong-Joon Yi, Dong Yeob Shin, Yeon-Keon Moon, Kyoung-Seok Son, Jun Hyung Lim, KwangSik Jeong* and Kwun-Bum Chung*,
{"title":"正偏压温度应力下氢扩散 InGaZnSnO TFT 中未占态的定量动态演化","authors":"Hyunmin Hong, Min Jung Kim, Dong-Joon Yi, Dong Yeob Shin, Yeon-Keon Moon, Kyoung-Seok Son, Jun Hyung Lim, KwangSik Jeong* and Kwun-Bum Chung*, ","doi":"10.1021/acsaelm.4c0143010.1021/acsaelm.4c01430","DOIUrl":null,"url":null,"abstract":"<p >Positive bias temperature stress (PBTS)-induced defects in self-aligned top-gate coplanar amorphous indium–gallium–zinc–tin oxide (a–IGZTO) thin-film transistors (TFTs) were quantitatively extracted as a function of hydrogen concentration. As the hydrogen concentration increased, the device properties and stability improved. As the stress time increased, the two decay constants that were extracted from the recovery of PBTS increased. Under PBTS, electrons were trapped in multiple defects simultaneously. Quantitative dynamic evolution of defect measurements showed that as the stress time increased, the activation energy and density of defects changed. As electrons moved to the dielectric, the density of shallow-level defects in the channel decreased, while the activation energy and density of deep-level defects increased. With a higher hydrogen concentration in the channel, the changes in defects were smaller. These findings indicate that hydrogen improves stability by passivating electron trap sites.</p>","PeriodicalId":4,"journal":{"name":"ACS Applied Energy Materials","volume":null,"pages":null},"PeriodicalIF":5.4000,"publicationDate":"2024-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Quantitative Dynamic Evolution of Unoccupied States in Hydrogen Diffused InGaZnSnO TFT under Positive Bias Temperature Stress\",\"authors\":\"Hyunmin Hong, Min Jung Kim, Dong-Joon Yi, Dong Yeob Shin, Yeon-Keon Moon, Kyoung-Seok Son, Jun Hyung Lim, KwangSik Jeong* and Kwun-Bum Chung*, \",\"doi\":\"10.1021/acsaelm.4c0143010.1021/acsaelm.4c01430\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Positive bias temperature stress (PBTS)-induced defects in self-aligned top-gate coplanar amorphous indium–gallium–zinc–tin oxide (a–IGZTO) thin-film transistors (TFTs) were quantitatively extracted as a function of hydrogen concentration. As the hydrogen concentration increased, the device properties and stability improved. As the stress time increased, the two decay constants that were extracted from the recovery of PBTS increased. Under PBTS, electrons were trapped in multiple defects simultaneously. Quantitative dynamic evolution of defect measurements showed that as the stress time increased, the activation energy and density of defects changed. As electrons moved to the dielectric, the density of shallow-level defects in the channel decreased, while the activation energy and density of deep-level defects increased. With a higher hydrogen concentration in the channel, the changes in defects were smaller. These findings indicate that hydrogen improves stability by passivating electron trap sites.</p>\",\"PeriodicalId\":4,\"journal\":{\"name\":\"ACS Applied Energy Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":5.4000,\"publicationDate\":\"2024-09-27\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Applied Energy Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsaelm.4c01430\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Energy Materials","FirstCategoryId":"88","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaelm.4c01430","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Quantitative Dynamic Evolution of Unoccupied States in Hydrogen Diffused InGaZnSnO TFT under Positive Bias Temperature Stress
Positive bias temperature stress (PBTS)-induced defects in self-aligned top-gate coplanar amorphous indium–gallium–zinc–tin oxide (a–IGZTO) thin-film transistors (TFTs) were quantitatively extracted as a function of hydrogen concentration. As the hydrogen concentration increased, the device properties and stability improved. As the stress time increased, the two decay constants that were extracted from the recovery of PBTS increased. Under PBTS, electrons were trapped in multiple defects simultaneously. Quantitative dynamic evolution of defect measurements showed that as the stress time increased, the activation energy and density of defects changed. As electrons moved to the dielectric, the density of shallow-level defects in the channel decreased, while the activation energy and density of deep-level defects increased. With a higher hydrogen concentration in the channel, the changes in defects were smaller. These findings indicate that hydrogen improves stability by passivating electron trap sites.
期刊介绍:
ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.