室温下光谱可调谐超快长波红外探测。

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2024-11-06 DOI:10.1021/acs.nanolett.4c03832
Tianyi Guo, Sayan Chandra, Arindam Dasgupta, Muhammad Waqas Shabbir, Aritra Biswas, Debashis Chanda
{"title":"室温下光谱可调谐超快长波红外探测。","authors":"Tianyi Guo, Sayan Chandra, Arindam Dasgupta, Muhammad Waqas Shabbir, Aritra Biswas, Debashis Chanda","doi":"10.1021/acs.nanolett.4c03832","DOIUrl":null,"url":null,"abstract":"<p><p>Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.</p>","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":null,"pages":null},"PeriodicalIF":9.6000,"publicationDate":"2024-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Spectrally Tunable Ultrafast Long Wave Infrared Detection at Room Temperature.\",\"authors\":\"Tianyi Guo, Sayan Chandra, Arindam Dasgupta, Muhammad Waqas Shabbir, Aritra Biswas, Debashis Chanda\",\"doi\":\"10.1021/acs.nanolett.4c03832\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.</p>\",\"PeriodicalId\":53,\"journal\":{\"name\":\"Nano Letters\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":9.6000,\"publicationDate\":\"2024-11-06\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nano Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1021/acs.nanolett.4c03832\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c03832","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

与低温冷却解决方案相比,室温长波红外(LWIR)探测器因其成本效益和操作简便而更受青睐。目前的非制冷型长波红外探测器(例如微测辐射热计)的性能受到灵敏度降低、响应时间慢以及缺乏动态光谱可调性等因素的限制。在这里,我们利用石墨烯的可调光学和电子特性,提出了一种具有高探测率和快速响应时间的高效室温近红外探测器。与光腔耦合的图案化石墨烯上的狄拉克质子增强了固有的弱光吸收。吸收的能量在非对称载流子生成环境下通过塞贝克效应转化为光电压。此外,还通过静电门控实现了 8-12 μm 长波红外波段的动态光谱可调谐性。所提出的探测平台为新一代基于石墨烯的非致冷长波红外光探测器铺平了道路,该探测器可广泛应用于分子传感、医疗诊断、军事、安全和太空等领域。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Spectrally Tunable Ultrafast Long Wave Infrared Detection at Room Temperature.

Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
期刊最新文献
Highly Monodisperse Stable Gold Nanorod Powder for Optical Sensor High-Performance Radiative Cooling Sunscreen Time-Domain-Filtered Terahertz Nanoscopy of Intrinsic Light–Matter Interactions Regulating Li2S Deposition and Accelerating Conversion Kinetics through Intracavity ZnS toward Low-Temperature Lithium–Sulfur Batteries Identifying the Role of Interfacial Long-Range Order in Regulating the Solid Electrolyte Interphase in Lithium Metal Batteries.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1