Keferson de A. Carvalho , Graiciany Barros , Matheus H.S. Araújo , Andre A. Campagnole dos Santos , Vitor Silva , Tiago Augusto Santiago Vieira , Rebeca Cabral Gonçalves
{"title":"关闭核燃料循环:类似 NuScale 反应堆的战略方法","authors":"Keferson de A. Carvalho , Graiciany Barros , Matheus H.S. Araújo , Andre A. Campagnole dos Santos , Vitor Silva , Tiago Augusto Santiago Vieira , Rebeca Cabral Gonçalves","doi":"10.1016/j.nucengdes.2024.113672","DOIUrl":null,"url":null,"abstract":"<div><div>The present study proposes the potential implementation of eight different closed fuel cycle strategies for a NuScale-like reactor core using its own spent fuel as a reusable source of fissile material for energy production. For that, the spent fuel composition after three burnup cycles of approximately 12 MWd/kgU of NuScale-like initial core and five years of cooling in a spent fuel pool was theoretically reprocessed by GANEX or UREX+ methods. After reprocessing, these two new fuel compositions were spiked in a mixture of thorium (Th) or depleted uranium (DpU), and afterwards inserted into specific batch positions of the core. Therefore, the proposed NuScale-like core configurations contain fuel assemblies loaded with conventional uranium-based fuel and others loaded with reprocessed fuel, resulting in the following combinations: UO<sub>2</sub> and GANEX spiked with Th, UO<sub>2</sub> and GANEX spiked with DpU, UO<sub>2</sub> and UREX+ spiked with Th, UO<sub>2</sub> and UREX+ spiked with DpU. The main idea is to comprehend the advantages of adopting the closed nuclear fuel cycle for a NuScale-like reactor by comparing the reference case and the cases containing reprocessed fuel. The results exhibited that all instances in which the core was simulated with reprocessed fuel improved the feedback coefficient, maximum excess of reactivity varying the boron concentration in the coolant, and power peak factor (PPF). Furthermore, the closed nuclear fuel strategies also demonstrated savings of about 17.50% in terms of separating work units (SWU) due to plutonium and uranium recycling, and a potential burnup extension of approximately 43%. The Serpent code version 2.1.32 developed by VTT and ENDF/B-VII.0 nuclear data library has been used to perform the simulations.</div></div>","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":null,"pages":null},"PeriodicalIF":16.4000,"publicationDate":"2024-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Closing the nuclear fuel cycle: Strategic approaches for NuScale-like reactor\",\"authors\":\"Keferson de A. Carvalho , Graiciany Barros , Matheus H.S. Araújo , Andre A. Campagnole dos Santos , Vitor Silva , Tiago Augusto Santiago Vieira , Rebeca Cabral Gonçalves\",\"doi\":\"10.1016/j.nucengdes.2024.113672\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The present study proposes the potential implementation of eight different closed fuel cycle strategies for a NuScale-like reactor core using its own spent fuel as a reusable source of fissile material for energy production. For that, the spent fuel composition after three burnup cycles of approximately 12 MWd/kgU of NuScale-like initial core and five years of cooling in a spent fuel pool was theoretically reprocessed by GANEX or UREX+ methods. After reprocessing, these two new fuel compositions were spiked in a mixture of thorium (Th) or depleted uranium (DpU), and afterwards inserted into specific batch positions of the core. Therefore, the proposed NuScale-like core configurations contain fuel assemblies loaded with conventional uranium-based fuel and others loaded with reprocessed fuel, resulting in the following combinations: UO<sub>2</sub> and GANEX spiked with Th, UO<sub>2</sub> and GANEX spiked with DpU, UO<sub>2</sub> and UREX+ spiked with Th, UO<sub>2</sub> and UREX+ spiked with DpU. The main idea is to comprehend the advantages of adopting the closed nuclear fuel cycle for a NuScale-like reactor by comparing the reference case and the cases containing reprocessed fuel. The results exhibited that all instances in which the core was simulated with reprocessed fuel improved the feedback coefficient, maximum excess of reactivity varying the boron concentration in the coolant, and power peak factor (PPF). Furthermore, the closed nuclear fuel strategies also demonstrated savings of about 17.50% in terms of separating work units (SWU) due to plutonium and uranium recycling, and a potential burnup extension of approximately 43%. 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Closing the nuclear fuel cycle: Strategic approaches for NuScale-like reactor
The present study proposes the potential implementation of eight different closed fuel cycle strategies for a NuScale-like reactor core using its own spent fuel as a reusable source of fissile material for energy production. For that, the spent fuel composition after three burnup cycles of approximately 12 MWd/kgU of NuScale-like initial core and five years of cooling in a spent fuel pool was theoretically reprocessed by GANEX or UREX+ methods. After reprocessing, these two new fuel compositions were spiked in a mixture of thorium (Th) or depleted uranium (DpU), and afterwards inserted into specific batch positions of the core. Therefore, the proposed NuScale-like core configurations contain fuel assemblies loaded with conventional uranium-based fuel and others loaded with reprocessed fuel, resulting in the following combinations: UO2 and GANEX spiked with Th, UO2 and GANEX spiked with DpU, UO2 and UREX+ spiked with Th, UO2 and UREX+ spiked with DpU. The main idea is to comprehend the advantages of adopting the closed nuclear fuel cycle for a NuScale-like reactor by comparing the reference case and the cases containing reprocessed fuel. The results exhibited that all instances in which the core was simulated with reprocessed fuel improved the feedback coefficient, maximum excess of reactivity varying the boron concentration in the coolant, and power peak factor (PPF). Furthermore, the closed nuclear fuel strategies also demonstrated savings of about 17.50% in terms of separating work units (SWU) due to plutonium and uranium recycling, and a potential burnup extension of approximately 43%. The Serpent code version 2.1.32 developed by VTT and ENDF/B-VII.0 nuclear data library has been used to perform the simulations.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.