量化氧化物异质结构中的极性天电离运动屏障

IF 5.8 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nanoscale Pub Date : 2024-11-12 DOI:10.1039/d4nr03686g
Lizhe Hu, Yuhui Huang, Yong Jun Wu, Zijian Hong
{"title":"量化氧化物异质结构中的极性天电离运动屏障","authors":"Lizhe Hu, Yuhui Huang, Yong Jun Wu, Zijian Hong","doi":"10.1039/d4nr03686g","DOIUrl":null,"url":null,"abstract":"Exotic polar topologies such as polar skyrmions have been widely observed in the ferroelectric superlattice system. The dynamic motion of the polar skyrmion under external forces holds promise for applications in advanced electronic devices such as race-track memory. Meanwhile, the polar skyrmion motion has proven to be challenging due to the strong skyrmion-skyrmion interaction and a lack of a mechanism similar to the spin-transfer torque. In this study, we have developed a nudged elastic band (NEB) method to quantify the polar skyrmion motion barrier along a specific trajectory. It is indicated that the skyrmion motion barrier can be significantly reduced with the reduction of the periodicity to 8 u.c., due to the large reduction of the skyrmion size. Moreover, this barrier can also be greatly reduced with a small external electric potential. Following the analysis, we further performed phase-field simulation to verify the collective motion of the polar skyrmion. We have demonstrated the skyrmion motion by applying a 5 μN mechanical force using a blame-shaped indenter with a periodicity of 8 unit cells, under an external applied voltage of 1.5 V. This study further paves the way for the design of the polar skyrmion-based electronic devices.","PeriodicalId":92,"journal":{"name":"Nanoscale","volume":"43 1","pages":""},"PeriodicalIF":5.8000,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Quantifying the polar skyrmion motion barrier in an oxide heterostructure\",\"authors\":\"Lizhe Hu, Yuhui Huang, Yong Jun Wu, Zijian Hong\",\"doi\":\"10.1039/d4nr03686g\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Exotic polar topologies such as polar skyrmions have been widely observed in the ferroelectric superlattice system. The dynamic motion of the polar skyrmion under external forces holds promise for applications in advanced electronic devices such as race-track memory. Meanwhile, the polar skyrmion motion has proven to be challenging due to the strong skyrmion-skyrmion interaction and a lack of a mechanism similar to the spin-transfer torque. In this study, we have developed a nudged elastic band (NEB) method to quantify the polar skyrmion motion barrier along a specific trajectory. It is indicated that the skyrmion motion barrier can be significantly reduced with the reduction of the periodicity to 8 u.c., due to the large reduction of the skyrmion size. Moreover, this barrier can also be greatly reduced with a small external electric potential. Following the analysis, we further performed phase-field simulation to verify the collective motion of the polar skyrmion. We have demonstrated the skyrmion motion by applying a 5 μN mechanical force using a blame-shaped indenter with a periodicity of 8 unit cells, under an external applied voltage of 1.5 V. This study further paves the way for the design of the polar skyrmion-based electronic devices.\",\"PeriodicalId\":92,\"journal\":{\"name\":\"Nanoscale\",\"volume\":\"43 1\",\"pages\":\"\"},\"PeriodicalIF\":5.8000,\"publicationDate\":\"2024-11-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nanoscale\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1039/d4nr03686g\",\"RegionNum\":3,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nanoscale","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d4nr03686g","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

在铁电超晶格系统中已广泛观察到极性天幕等奇异的极性拓扑结构。极性天幕在外力作用下的动态运动有望应用于赛道存储器等先进电子设备中。与此同时,由于极性天融子与天融子之间存在很强的相互作用,而且缺乏类似于自旋转移力矩的机制,因此极性天融子的运动被证明具有挑战性。在这项研究中,我们开发了一种裸弹带(NEB)方法来量化沿特定轨迹的极性天融运动障碍。结果表明,随着周期性减小到 8 u.c.,天离子运动障碍会显著减小,这是由于天离子尺寸的大幅减小。此外,小的外部电势也能大大降低这一障碍。在分析之后,我们进一步进行了相场模拟,以验证极性天融子的集体运动。在 1.5 V 的外加电压下,我们使用周期为 8 个单元格的责状压头施加了 5 μN 的机械力,证明了天空离子的运动。这项研究为设计基于极性天电离子的电子器件进一步铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Quantifying the polar skyrmion motion barrier in an oxide heterostructure
Exotic polar topologies such as polar skyrmions have been widely observed in the ferroelectric superlattice system. The dynamic motion of the polar skyrmion under external forces holds promise for applications in advanced electronic devices such as race-track memory. Meanwhile, the polar skyrmion motion has proven to be challenging due to the strong skyrmion-skyrmion interaction and a lack of a mechanism similar to the spin-transfer torque. In this study, we have developed a nudged elastic band (NEB) method to quantify the polar skyrmion motion barrier along a specific trajectory. It is indicated that the skyrmion motion barrier can be significantly reduced with the reduction of the periodicity to 8 u.c., due to the large reduction of the skyrmion size. Moreover, this barrier can also be greatly reduced with a small external electric potential. Following the analysis, we further performed phase-field simulation to verify the collective motion of the polar skyrmion. We have demonstrated the skyrmion motion by applying a 5 μN mechanical force using a blame-shaped indenter with a periodicity of 8 unit cells, under an external applied voltage of 1.5 V. This study further paves the way for the design of the polar skyrmion-based electronic devices.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
期刊最新文献
Holey etching strategy of siloxene nanosheets to improve the rate performance of photo-assisted Li–O2 batteries Enantiomorphic single component conducting nickel(II) and platinum(II) bis(diethyl-dddt) crystalline complexes† Facile synthesis of in situ carbon-coated CoS2 micro/nano-spheres as high-performance anode materials for sodium-ion batteries A layered Janus Metastructure for multi-physical detection based on second harmonic wave Correction: Cytomembrane-mimicking nanocarriers with a scaffold consisting of a CD44-targeted endogenous component for effective asparaginase supramolecule delivery
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1