超轻型 RGO 基气凝胶的均匀填充工艺,在芳纶蜂窝中实现宽带微波吸收

IF 3.5 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Journal of Materials Science Pub Date : 2024-11-06 DOI:10.1007/s10853-024-10335-x
Hongfang Qiu, Jian Peng, Weiwei Xu, Xiong Fang, Junyu Lu, Xiaochuang Di, Zhao Lu, Yang Chen, Huawei Zou
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引用次数: 0

摘要

如果没有可靠的机械支撑结构,在实际航空航天应用中使用微波吸收(MA)材料将面临挑战。然而,在芳纶蜂窝结构中实现较宽的有效吸收带宽(EAB)且重量不变,对于微波吸收材料在航空航天领域的实际应用至关重要。为应对这一挑战,本研究提出将多孔碳泡沫和高结构强度蜂窝相结合,通过碳泡沫吸收和蜂窝结构的协同效应,在结构装置中实现宽带微波吸收。通过冷冻干燥实现了超轻还原GO气凝胶的均匀填充过程,解决了传统吸波材料在蜂窝中分散不均匀和填充不完全的问题。对填充浓度和还原工艺进行了进一步优化和综合评价。冷冻干燥工艺与填充不同浓度 GO 的化学还原蜂窝样品相结合,均表现出宽带吸收性能。在 15 毫米的特定标准蜂窝厚度下,均匀填充 0.1% 至 0.3% GO 的蜂窝样品在 2-3 GHz、8-9 GHz 和 15 GHz 附近显示出三重共振峰,有效吸收峰值均低于 - 10 dB。此外,透明波蜂窝壁与蜂窝材料的结合增强了整体阻抗匹配,使填充 0.2% 冻干和还原 GO 的蜂窝样品的 EAB 进一步提高到 10.53 GHz。CST 仿真数据证实,蜂窝样品中的损耗源于均匀传导损耗,电场稳定地进入蜂窝内部。这种基于冻干技术快速高效填充均匀 RGO 的方法为芳纶蜂窝实现宽带微波吸收提供了一种新途径,在航空航天隐身领域具有巨大的发展潜力。
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Uniform filling process of ultra-lightweight RGO-based aerogel for achieving broadband microwave absorption in aramid honeycomb

The use of microwave absorption (MA) materials in practical aerospace applications would be challenging without a dependable mechanical support structure. However, achieving a wide effective absorption bandwidth (EAB) in aramid honeycomb structures at low weight gain is crucial for the practical aerospace applications of MA materials. To address this challenge, this study proposes a combination of porous carbon foam and high structural strength honeycomb to achieve broadband microwave absorption in structural devices through the synergistic effect of carbon foam absorption and honeycomb structure. The uniform filling process of ultra-lightweight reduced GO aerogel is achieved through freeze-drying, solving the issues of uneven dispersion and incomplete filling of traditional absorbers in honeycombs. Further optimization and comprehensive evaluation of filling concentration and reduction process were carried out. The freeze-drying process combined with chemically reduced honeycomb samples filled with different concentrations of GO all exhibit broadband absorption performance. At a specific standard honeycomb thickness of 15 mm, uniformly filled honeycomb samples with 0.1 to 0.3% GO exhibit triple resonance peaks near 2–3 GHz, 8–9 GHz, and 15 GHz, with effective absorption peaks all below − 10 dB. Moreover, the incorporation of transparent wave honeycomb walls in conjunction with honeycomb materials enhances the overall impedance matching, leading to a further improvement in the EAB to 10.53 GHz for the honeycomb sample filled with 0.2% freeze-dried and reduced GO. CST simulation data confirms that the loss in the honeycomb samples originates from uniform conduction loss, and the electric field stably enters the interior of the honeycomb. This approach, based on the rapid and efficient filling of uniform RGO by freeze-drying, provides a new way to achieve broadband microwave absorption in aramid honeycombs and has significant potential for development in the field of aerospace stealth.

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来源期刊
Journal of Materials Science
Journal of Materials Science 工程技术-材料科学:综合
CiteScore
7.90
自引率
4.40%
发文量
1297
审稿时长
2.4 months
期刊介绍: The Journal of Materials Science publishes reviews, full-length papers, and short Communications recording original research results on, or techniques for studying the relationship between structure, properties, and uses of materials. The subjects are seen from international and interdisciplinary perspectives covering areas including metals, ceramics, glasses, polymers, electrical materials, composite materials, fibers, nanostructured materials, nanocomposites, and biological and biomedical materials. The Journal of Materials Science is now firmly established as the leading source of primary communication for scientists investigating the structure and properties of all engineering materials.
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