Shezhan Liu , Yi Zhang , Lei Yuan , Siyu Xu , Lanlan Jiang , Yuechao Zhao , Yongchen Song
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The optimized EGR injection schemes were proposed, in which the first stage was displaced by N<sub>2</sub> or CO<sub>2</sub> mixtures as booster gas, while the second stage was displaced by CO<sub>2</sub> to improve CH<sub>4</sub> recovery and CO<sub>2</sub> sequestration efficiency as well as to reduce CO<sub>2</sub> capture costs. Both N<sub>2</sub> and flue gas were found to perform well as booster gas in the gaseous state. The highest CH<sub>4</sub> recovery efficiency of 36.05% and the highest CO<sub>2</sub> sequestration efficiency of 21.31% were obtained for N<sub>2</sub> as booster gas in dry rock core due to the overall improved sweep efficiency and the barricade effect of N<sub>2</sub>. Whereas, the flue gas as booster gas had better performance under supercritical conditions with the highest recovery efficiency of 36.69%. In addition, it was found that the dispersion coefficients of the optimized injection schemes became larger due to the pipeline entry/exit effects. Due to the dissolution of CO<sub>2</sub> into connate water, the optimized scheme had the best results in CH<sub>4</sub> recovery and CO<sub>2</sub> sequestration with flue gas as the booster gas, improving by 20.5% and 13.5%, respectively, compared to the conventional CO<sub>2</sub> injection scheme.</div></div>","PeriodicalId":100578,"journal":{"name":"Geoenergy Science and Engineering","volume":"244 ","pages":"Article 213508"},"PeriodicalIF":0.0000,"publicationDate":"2024-11-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Experimental study of optimized injection schemes for enhanced gas recovery and carbon sequestration\",\"authors\":\"Shezhan Liu , Yi Zhang , Lei Yuan , Siyu Xu , Lanlan Jiang , Yuechao Zhao , Yongchen Song\",\"doi\":\"10.1016/j.geoen.2024.213508\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>To reduce the carbon capture costs in CO<sub>2</sub> enhanced gas recovery (EGR) process, three types of displacing fluids, pure CO<sub>2</sub>, flue gas and gas-altering gas, were used in the conventional injection mode for experimental comparison. It was found that pure CO<sub>2</sub> had the highest recovery efficiency and the smallest dispersion coefficient at supercritical state. The dispersion coefficients of the three displacing fluids became larger with increasing water saturation. The optimized EGR injection schemes were proposed, in which the first stage was displaced by N<sub>2</sub> or CO<sub>2</sub> mixtures as booster gas, while the second stage was displaced by CO<sub>2</sub> to improve CH<sub>4</sub> recovery and CO<sub>2</sub> sequestration efficiency as well as to reduce CO<sub>2</sub> capture costs. Both N<sub>2</sub> and flue gas were found to perform well as booster gas in the gaseous state. The highest CH<sub>4</sub> recovery efficiency of 36.05% and the highest CO<sub>2</sub> sequestration efficiency of 21.31% were obtained for N<sub>2</sub> as booster gas in dry rock core due to the overall improved sweep efficiency and the barricade effect of N<sub>2</sub>. Whereas, the flue gas as booster gas had better performance under supercritical conditions with the highest recovery efficiency of 36.69%. In addition, it was found that the dispersion coefficients of the optimized injection schemes became larger due to the pipeline entry/exit effects. Due to the dissolution of CO<sub>2</sub> into connate water, the optimized scheme had the best results in CH<sub>4</sub> recovery and CO<sub>2</sub> sequestration with flue gas as the booster gas, improving by 20.5% and 13.5%, respectively, compared to the conventional CO<sub>2</sub> injection scheme.</div></div>\",\"PeriodicalId\":100578,\"journal\":{\"name\":\"Geoenergy Science and Engineering\",\"volume\":\"244 \",\"pages\":\"Article 213508\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-11-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Geoenergy Science and Engineering\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2949891024008789\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"0\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Geoenergy Science and Engineering","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2949891024008789","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"0","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0
摘要
为降低二氧化碳强化气体回收(EGR)工艺中的碳捕集成本,在常规注入模式下,使用了纯二氧化碳、烟道气和改气气体三种置换流体进行实验比较。结果发现,在超临界状态下,纯 CO2 的回收效率最高,分散系数最小。三种置换流体的分散系数随着水饱和度的增加而变大。提出了优化的 EGR 喷射方案,其中第一阶段用 N2 或 CO2 混合物作为增压气体进行置换,第二阶段用 CO2 进行置换,以提高 CH4 回收率和 CO2 封存效率,并降低 CO2 捕获成本。作为气态增压气体,N2 和烟道气的性能都很好。在干燥岩芯中,N2 作为增压气体的 CH4 回收效率最高,达到 36.05%,CO2 封存效率最高,达到 21.31%,这主要归功于 N2 全面提高的扫气效率和屏障效应。而烟道气作为增压气体在超临界条件下性能更好,回收效率最高,达到 36.69%。此外,研究还发现,由于管道出入口效应,优化注入方案的分散系数变大。由于二氧化碳溶解到涵养水中,以烟道气为增压气体的优化方案在甲烷回收和二氧化碳封存方面效果最佳,与传统的二氧化碳注入方案相比,分别提高了 20.5% 和 13.5%。
Experimental study of optimized injection schemes for enhanced gas recovery and carbon sequestration
To reduce the carbon capture costs in CO2 enhanced gas recovery (EGR) process, three types of displacing fluids, pure CO2, flue gas and gas-altering gas, were used in the conventional injection mode for experimental comparison. It was found that pure CO2 had the highest recovery efficiency and the smallest dispersion coefficient at supercritical state. The dispersion coefficients of the three displacing fluids became larger with increasing water saturation. The optimized EGR injection schemes were proposed, in which the first stage was displaced by N2 or CO2 mixtures as booster gas, while the second stage was displaced by CO2 to improve CH4 recovery and CO2 sequestration efficiency as well as to reduce CO2 capture costs. Both N2 and flue gas were found to perform well as booster gas in the gaseous state. The highest CH4 recovery efficiency of 36.05% and the highest CO2 sequestration efficiency of 21.31% were obtained for N2 as booster gas in dry rock core due to the overall improved sweep efficiency and the barricade effect of N2. Whereas, the flue gas as booster gas had better performance under supercritical conditions with the highest recovery efficiency of 36.69%. In addition, it was found that the dispersion coefficients of the optimized injection schemes became larger due to the pipeline entry/exit effects. Due to the dissolution of CO2 into connate water, the optimized scheme had the best results in CH4 recovery and CO2 sequestration with flue gas as the booster gas, improving by 20.5% and 13.5%, respectively, compared to the conventional CO2 injection scheme.