Tinglu Song , Huaqiang Zhu , Chunlin Zhang , Yan Chen , Fan Xu , Mengzhan Ge , Zhaoyu Xue , Xiaodong Li , Meishuai Zou
{"title":"通过碘化铋改进复合网络,实现高效冰核应用","authors":"Tinglu Song , Huaqiang Zhu , Chunlin Zhang , Yan Chen , Fan Xu , Mengzhan Ge , Zhaoyu Xue , Xiaodong Li , Meishuai Zou","doi":"10.1016/j.surfin.2024.105404","DOIUrl":null,"url":null,"abstract":"<div><div>The urgent demand for electricity requires more safe energy transportation. AgI-based weather modification agents are commonly employed to facilitate ice nucleation and remove the undesirable glaze icing to suppress the negative effects of natural disasters. However, the intrinsic nucleation potency of AgI strictly limits its further improvement. Here, a hexagonal BiI<sub>3</sub> was added in AgI-based agents. The chemical interactions of BiI<sub>3</sub> and precursors optimize the crystallization of the polymer composite, leading to an oriented composite network. In addition, BiI<sub>3</sub> could alter the structure and morphology of the combustion products, therefore creating more possible heterogeneous nuclei sites. The resultant BiI<sub>3</sub>-modified AgI-based weather modification agent exhibits an ice nucleation ∼ 10<sup>14</sup>, which is nearly ten times higher than the sample without AgI-BiI<sub>3</sub>, leading to a 71.21 % enhancement of deicing efficiency compared to AgI sample. Our results indicate the effectiveness of BiI<sub>3</sub> dopant to improve both nucleation and deicing performance for weather modification applications.</div></div>","PeriodicalId":22081,"journal":{"name":"Surfaces and Interfaces","volume":"55 ","pages":"Article 105404"},"PeriodicalIF":5.7000,"publicationDate":"2024-11-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Improved composite network via bismuth iodide for efficient ice-nucleating application\",\"authors\":\"Tinglu Song , Huaqiang Zhu , Chunlin Zhang , Yan Chen , Fan Xu , Mengzhan Ge , Zhaoyu Xue , Xiaodong Li , Meishuai Zou\",\"doi\":\"10.1016/j.surfin.2024.105404\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The urgent demand for electricity requires more safe energy transportation. AgI-based weather modification agents are commonly employed to facilitate ice nucleation and remove the undesirable glaze icing to suppress the negative effects of natural disasters. However, the intrinsic nucleation potency of AgI strictly limits its further improvement. Here, a hexagonal BiI<sub>3</sub> was added in AgI-based agents. The chemical interactions of BiI<sub>3</sub> and precursors optimize the crystallization of the polymer composite, leading to an oriented composite network. In addition, BiI<sub>3</sub> could alter the structure and morphology of the combustion products, therefore creating more possible heterogeneous nuclei sites. The resultant BiI<sub>3</sub>-modified AgI-based weather modification agent exhibits an ice nucleation ∼ 10<sup>14</sup>, which is nearly ten times higher than the sample without AgI-BiI<sub>3</sub>, leading to a 71.21 % enhancement of deicing efficiency compared to AgI sample. Our results indicate the effectiveness of BiI<sub>3</sub> dopant to improve both nucleation and deicing performance for weather modification applications.</div></div>\",\"PeriodicalId\":22081,\"journal\":{\"name\":\"Surfaces and Interfaces\",\"volume\":\"55 \",\"pages\":\"Article 105404\"},\"PeriodicalIF\":5.7000,\"publicationDate\":\"2024-11-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Surfaces and Interfaces\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2468023024015608\",\"RegionNum\":2,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Surfaces and Interfaces","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2468023024015608","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Improved composite network via bismuth iodide for efficient ice-nucleating application
The urgent demand for electricity requires more safe energy transportation. AgI-based weather modification agents are commonly employed to facilitate ice nucleation and remove the undesirable glaze icing to suppress the negative effects of natural disasters. However, the intrinsic nucleation potency of AgI strictly limits its further improvement. Here, a hexagonal BiI3 was added in AgI-based agents. The chemical interactions of BiI3 and precursors optimize the crystallization of the polymer composite, leading to an oriented composite network. In addition, BiI3 could alter the structure and morphology of the combustion products, therefore creating more possible heterogeneous nuclei sites. The resultant BiI3-modified AgI-based weather modification agent exhibits an ice nucleation ∼ 1014, which is nearly ten times higher than the sample without AgI-BiI3, leading to a 71.21 % enhancement of deicing efficiency compared to AgI sample. Our results indicate the effectiveness of BiI3 dopant to improve both nucleation and deicing performance for weather modification applications.
期刊介绍:
The aim of the journal is to provide a respectful outlet for ''sound science'' papers in all research areas on surfaces and interfaces. We define sound science papers as papers that describe new and well-executed research, but that do not necessarily provide brand new insights or are merely a description of research results.
Surfaces and Interfaces publishes research papers in all fields of surface science which may not always find the right home on first submission to our Elsevier sister journals (Applied Surface, Surface and Coatings Technology, Thin Solid Films)