粘弹性流体中通过粘指法和弹性压裂侵入气体的速度场特征比较。

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Soft Matter Pub Date : 2024-11-26 DOI:10.1039/d4sm00982g
Zhao Jin, Yixuan Hou, Xinzhe Que, Yongchao Zhou, Yiping Zhang
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引用次数: 0

摘要

粘指状(VF)和弹性断裂(EFr)是气体侵入复杂流体时的普遍现象。在这项研究中,通过在矩形海尔-肖电池中进行单点注入,将压缩氮气注入一种名为镁锂硅酸盐(MLPS)悬浮液的复杂流体中。在气体通过 VF 侵入 MLPS 悬浮液的情况下,受影响区域仅限于分裂后独立生长的指尖。在受影响区域内,速度主要平行于手指的生长方向,而垂直分量主要分布在整个气泡的外侧,且范围较为有限。气液界面可分为移动边界和静止边界,其中移动边界的长度远小于气泡的周长。在运动边界上,与生长方向平行的速度分量在影响范围和影响程度上都明显大于垂直分量。速度方向与生长方向之间的夹角集中在一个很小的范围内,显示出速度之间显著的正相关性。相反,当气泡通过 EFr 侵入时,受干扰的区域更大,平行速度分量主要位于气泡顶端,而垂直分量则呈 "蝴蝶 "状分布在气泡中部。移动边界长度与气泡周长相当。在移动边界上,垂直分量产生了不可忽略的影响,并且包含的角度分布更加均匀,从而导致速度之间出现明显的负相关。根据速度场的上述特点,提出了受影响面积比、移动边界长度与周长比、速度分量比、均匀性系数、相对相关长度等定量指标。基于速度场,这些指标在区分复杂流体中观察到的两种不同入侵模式方面显示出普遍适用性。
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Comparison of velocity field characteristics of gas invasion via viscous fingering and elastic fracturing in visco-elasto-plastic fluids.

Viscous fingering (VF) and elastic fracture (EFr) are prevalent phenomena when gas invades into complex fluids. In this study, compressed nitrogen gas was injected into a complex fluid called magnesium lithium phyllosilicate (MLPS) suspension through a single-point injection in a rectangular Hele-Shaw cell. In the case of gas invasion into the MLPS suspension via VF, the affected area is confined to the tips of the independently growing fingers after splitting. Within the affected region, the velocity is primarily parallel to the growth direction of fingers, while the perpendicular component is mainly distributed on the outer sides of the whole bubble and within a more limited range. The gas-liquid interface can be divided into moving and static boundaries, where the length of the moving boundary is much smaller than the perimeter of the bubble. On the moving boundary, the parallel velocity component to the growth direction is significantly greater than the perpendicular component in terms of both the influence range and magnitude. The included angles between the velocity direction and the growth direction are concentrated within a narrow range, showing a significant positive correlation among the velocities. Conversely, when a bubble invades via EFr, the disturbed area is larger, with the parallel velocity component primarily located at the tip and the perpendicular component distributed in a "butterfly" shape around the middle of the bubble. The moving boundary length is comparable to the bubble perimeter. On the moving boundary, the perpendicular component exerts a non-negligible influence, and the distribution of included angles is more uniform, resulting in a significant negative correlation among the velocities. Based on the above characteristics of the velocity field, quantitative indicators, such as the ratio of the affected area, the ratio of moving boundary length to the perimeter, the velocity component ratio, the coefficient of uniformity, and the relative correlation length, are proposed. Based on the velocity field, these indicators demonstrate universal applicability in distinguishing between the two different invasion patterns observed in complex fluids.

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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Where physics meets chemistry meets biology for fundamental soft matter research.
期刊最新文献
Back cover Collective motion of energy depot active disks. Comparison of velocity field characteristics of gas invasion via viscous fingering and elastic fracturing in visco-elasto-plastic fluids. Composite of knitted fabric and soft matrix. I. Crack growth in the course direction. Divalent cation effects in the glass transition of poly(diallyldimethylammonium)-poly(styrene sulfonate) polyelectrolyte complexes.
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