北部三个选定地区地下水中的氡污染、风险评估及其空间分布

IF 3.4 2区 地球科学 Q1 GEOCHEMISTRY & GEOPHYSICS Journal of Geochemical Exploration Pub Date : 2024-11-22 DOI:10.1016/j.gexplo.2024.107644
Said Muhammad , Rizwan Ullah , Sehrish Amin , Ashfaq Ahmad
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引用次数: 0

摘要

氡(222Rn)在环境中无处不在,会对生物的健康造成严重威胁。地下水是该地区 300 万人饮用和生活用水的主要来源。本研究旨在调查地下水中 222Rn 的浓度和相关健康风险。为此,使用 RAD7 检测器(美国 Durridge 公司)检测了地下水中 222Rn 的浓度。222Rn 的平均浓度在下迪尔区最高,为 10.8 ± 3.6 Bq/L,在上迪尔区最低,为 6.39 ± 0.98 Bq/L。不过,下迪尔 30% 采样点的 222Rn 浓度高于 11.1 Bq/L 的建议水平。这项研究评估了不同年龄段的人因摄入地下水中的 222Rn 而面临的潜在非致癌风险和估计终生致癌风险 (ELCR)。结果显示,婴儿的年均总暴露剂量(EwTotal)值为 43.7 ± 10.2、25.2 ± 3.15、27.0 ± 1.68 μSv/a,儿童为 33.5 ± 7.80、19.3 ± 2.42、20.1 ± 1.68 μSv/a。在下迪尔、上迪尔和吉德拉尔地区,成人(32.3 ± 7.52、18.6 ± 2.33、20.0 ± 1.24 μSv/a)和儿童(33.5 ± 7.80、19.3 ± 2.42、20.1 ± 1.29 μSv/a)分别摄入地下水。婴儿更容易因地下水中的 222Rn 污染而出现健康问题。222Rn 浓度与所研究的地下水中各种物理化学参数的相关性较弱。
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Radon contamination, risk evaluation, and their spatial distribution in groundwater of three selected northern districts
Radon (222Rn) has a ubiquitous nature in the environment and can pose serious health threats to living beings. Groundwater is the primary source of drinking and domestic uses for >3 million people in the area. The current study was conducted for investigation of groundwater for the 222Rn concentration and associated health risks. For that purpose, the groundwater was examined for 222Rn concentration using the RAD7 detector (Durridge Company, USA). Average concentrations of 222Rn were highest at 10.8 ± 3.6 Bq/L in the Lower Dir district and lowest at 6.39 ± 0.98 Bq/L in the Upper Dir. The average concentration of 222Rn was found below the threshold limit set by the US Environmental Protection Agency (USEPA) and the World Health Organization (WHO). However, the concentration in 30 % of sampling sites in the Lower Dir showed 222Rn concentrations higher than a recommended level of 11.1 Bq/L. This study evaluated the potential non-cancer risk and estimated lifetime cancer risk (ELCR) of various age groups via 222Rn consumption in groundwater. The results showed´s total annual mean exposure doses (EwTotal) values for infant of 43.7 ± 10.2, 25.2 ± 3.15, 27.0 ± 1.68 μSv/a, children 33.5 ± 7.80, 19.3 ± 2.42, 20.1 ± 1.29 μSv/a), and adults (32.3 ± 7.52, 18.6 ± 2.33, 20.0 ± 1.24 μSv/a) via groundwater intake in Lower Dir, Upper Dir, and Chitral districts, respectively. Infants showed higher vulnerability to health issues due to 222Rn contamination in groundwater. 222Rn concentrations showed a weak correlation with various studied physicochemical parameters in the groundwater.
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来源期刊
Journal of Geochemical Exploration
Journal of Geochemical Exploration 地学-地球化学与地球物理
CiteScore
7.40
自引率
7.70%
发文量
148
审稿时长
8.1 months
期刊介绍: Journal of Geochemical Exploration is mostly dedicated to publication of original studies in exploration and environmental geochemistry and related topics. Contributions considered of prevalent interest for the journal include researches based on the application of innovative methods to: define the genesis and the evolution of mineral deposits including transfer of elements in large-scale mineralized areas. analyze complex systems at the boundaries between bio-geochemistry, metal transport and mineral accumulation. evaluate effects of historical mining activities on the surface environment. trace pollutant sources and define their fate and transport models in the near-surface and surface environments involving solid, fluid and aerial matrices. assess and quantify natural and technogenic radioactivity in the environment. determine geochemical anomalies and set baseline reference values using compositional data analysis, multivariate statistics and geo-spatial analysis. assess the impacts of anthropogenic contamination on ecosystems and human health at local and regional scale to prioritize and classify risks through deterministic and stochastic approaches. Papers dedicated to the presentation of newly developed methods in analytical geochemistry to be applied in the field or in laboratory are also within the topics of interest for the journal.
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