析氧反应的活性-稳定性关系。

IF 9.1 Q2 CHEMISTRY, PHYSICAL ACS Materials Au Pub Date : 2024-11-15 eCollection Date: 2025-01-08 DOI:10.1021/acsmaterialsau.4c00086
Wonchul Park, Dong Young Chung
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引用次数: 0

摘要

析氧反应(OER)是各种可持续能源技术的关键过程。尽管催化剂的发展取得了实质性进展,但OER催化剂的实际应用仍然受到平衡高催化活性和长期稳定性的持续挑战的阻碍。我们探讨了活动和稳定性之间经常观察到的反向趋势,借鉴了实验和理论研究的关键见解。特别关注不同电极的性能及其在一系列电化学条件下与酸性和碱性介质的相互作用。本文整合了最新进展,为理解活性-稳定性关系的机制提供了一个全面的框架,为合理设计下一代OER催化剂提供了策略,成功地满足了活性和耐久性的双重要求。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Activity-Stability Relationships in Oxygen Evolution Reaction.

The oxygen evolution reaction (OER) is a critical process in various sustainable energy technologies. Despite substantial progress in catalyst development, the practical application of OER catalysts remains hindered by the ongoing challenge of balancing high catalytic activity with long-term stability. We explore the inverse trends often observed between activity and stability, drawing on key insights from both experimental and theoretical studies. Special focus is placed on the performance of different electrodes and their interaction with acidic and alkaline media across a range of electrochemical conditions. This Perspective integrates recent advancements to present a thorough framework for understanding the mechanisms underlying the activity-stability relationship, offering strategies for the rational design of next-generation OER catalysts that successfully meet the dual demands of activity and durability.

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来源期刊
ACS Materials Au
ACS Materials Au 材料科学-
CiteScore
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期刊介绍: ACS Materials Au is an open access journal publishing letters articles reviews and perspectives describing high-quality research at the forefront of fundamental and applied research and at the interface between materials and other disciplines such as chemistry engineering and biology. Papers that showcase multidisciplinary and innovative materials research addressing global challenges are especially welcome. Areas of interest include but are not limited to:Design synthesis characterization and evaluation of forefront and emerging materialsUnderstanding structure property performance relationships and their underlying mechanismsDevelopment of materials for energy environmental biomedical electronic and catalytic applications
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