Pb中扁平带\(_2\) Bi \(_2\) O \(_7\):迈向“扁平电子学”的新一步

IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Journal of Superconductivity and Novel Magnetism Pub Date : 2025-01-15 DOI:10.1007/s10948-025-06903-0
Izumi Hase
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引用次数: 0

摘要

在具有强几何挫折的晶格上的电子模型(平带模型)中,电子的能带色散会消失,导致所谓的平带。众所周知,平带是各种有趣的物理性质出现的平台。然而,在实际材料中实现平带仍然是一项具有挑战性的任务。在本文中,我们报告了平带模型在氧化焦绿盐Pb \(_2\) Bi \(_2\) O \(_7\)中近似成立,正如第一线原理计算所证明的那样。此外,我们提出,在平带系统的两个关键参数——平带宽度和载流子密度中,后者可以通过利用固溶体Pb \(_2\) (Sb,Bi) \(_2\) O \(_7\)有选择性地进行近似控制。这一发现代表了迈向“平面电子学”的新一步,“平面电子学”是一个专注于控制平面带系统的领域。
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Flat Bands in Pb\(_2\)Bi\(_2\)O\(_7\): A New Step Towards the Realization of “Flatronics”

In electronic models on lattices with strong geometric frustration (flat band models), the band dispersion of electrons can vanish, resulting in what is known as a flat band. Flat bands are known to serve as a platform for the emergence of various intriguing physical properties. Realizing flat bands in actual materials, however, remains a challenging task. In this paper, we report that the flat band model approximately holds in the pyrochlore oxide Pb\(_2\)Bi\(_2\)O\(_7\), as demonstrated by first-principles calculations. Furthermore, we propose that, among the two key parameters in flat band systems—the flat band width and the carrier density—the latter can be selectively controlled, approximately, by utilizing the solid solution Pb\(_2\)(Sb,Bi)\(_2\)O\(_7\). This finding represents a new step toward “flatronics,” a field focused on controlling flat band systems.

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来源期刊
Journal of Superconductivity and Novel Magnetism
Journal of Superconductivity and Novel Magnetism 物理-物理:凝聚态物理
CiteScore
3.70
自引率
11.10%
发文量
342
审稿时长
3.5 months
期刊介绍: The Journal of Superconductivity and Novel Magnetism serves as the international forum for the most current research and ideas in these fields. This highly acclaimed journal publishes peer-reviewed original papers, conference proceedings and invited review articles that examine all aspects of the science and technology of superconductivity, including new materials, new mechanisms, basic and technological properties, new phenomena, and small- and large-scale applications. Novel magnetism, which is expanding rapidly, is also featured in the journal. The journal focuses on such areas as spintronics, magnetic semiconductors, properties of magnetic multilayers, magnetoresistive materials and structures, magnetic oxides, etc. Novel superconducting and magnetic materials are complex compounds, and the journal publishes articles related to all aspects their study, such as sample preparation, spectroscopy and transport properties as well as various applications.
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