1T-TaS2中不同堆积面畴壁附近电子态的空间演化

IF 2.4 4区 物理与天体物理 Q3 PHYSICS, CONDENSED MATTER Solid State Communications Pub Date : 2025-03-01 Epub Date: 2024-12-19 DOI:10.1016/j.ssc.2024.115810
Yuto Nakashima , Atsushi Nomura , Hideaki Sakata
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引用次数: 0

摘要

1T-TaS2是一种准二维层状材料,在低温下具有不同能隙的两个不同的绝缘表面。这些不同绝缘状态的原因已经在文献中研究了由相称电荷密度波二聚化引起的带绝缘状态或莫特绝缘状态。为了阐明这两种绝缘态的特征,我们利用扫描隧道显微镜和扫描隧道光谱观察了v -取代1T-TaS2表面近畴壁电态的空间演化。在两个表面上,我们观察到间隙结构的崩溃,并伴随着在畴壁处出现间隙态。我们发现这些间隙态的衰减长度随表面类型的不同而变化。在小间隙表面观测到的短衰减长度与第一性原理计算结果吻合得很好。
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Spatial evolution of the electronic states near a domain wall on different stacking surfaces in 1T-TaS2
1T-TaS2 is a quasi-two-dimensional layered material that exhibits two distinct insulating surfaces with varying energy gaps at low temperature. The cause of these different insulating states has been investigated in the context of a band-insulating state resulting from the dimerization of a commensurate charge-density wave or a Mott-insulating state, in literatures. To elucidate the characteristics of these two insulating states, we observed the spatial evolution of the electric states near a domain wall on both surfaces of V-substituted 1T-TaS2 by scanning tunneling microscopy and scanning tunneling spectroscopy. On both surfaces, we observed the collapse of gap structures, accompanied by the emergence of in-gap states at the domain wall. We found that the decay lengths of these in-gap states varied depending on the surface type. The short decay length observed on the small-gap surface is in good agreement of the first principles calculation.
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来源期刊
Solid State Communications
Solid State Communications 物理-物理:凝聚态物理
CiteScore
3.40
自引率
4.80%
发文量
287
审稿时长
51 days
期刊介绍: Solid State Communications is an international medium for the publication of short communications and original research articles on significant developments in condensed matter science, giving scientists immediate access to important, recently completed work. The journal publishes original experimental and theoretical research on the physical and chemical properties of solids and other condensed systems and also on their preparation. The submission of manuscripts reporting research on the basic physics of materials science and devices, as well as of state-of-the-art microstructures and nanostructures, is encouraged. A coherent quantitative treatment emphasizing new physics is expected rather than a simple accumulation of experimental data. Consistent with these aims, the short communications should be kept concise and short, usually not longer than six printed pages. The number of figures and tables should also be kept to a minimum. Solid State Communications now also welcomes original research articles without length restrictions. The Fast-Track section of Solid State Communications is the venue for very rapid publication of short communications on significant developments in condensed matter science. The goal is to offer the broad condensed matter community quick and immediate access to publish recently completed papers in research areas that are rapidly evolving and in which there are developments with great potential impact.
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